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Interpreting Chiral Nanophotonic Spectra: The Plasmonic Born–Kuhn Model
Abstract
One of the most intuitive ways to classically understand the generation of natural optical activity in chiral media is provided by the coupled oscillator model of Born and Kuhn consisting of two identical, vertically displaced, coupled oscillators. We experimentally realize and discuss its exact plasmonic analog in a system of corner-stacked gold nanorods. In particular, we analyze the arising circular dichroism and optical rotatory spectra in terms of hybridized electromagnetic modes and retardation. Specifically, we demonstrate how tuning the vertical distance between the nanorods can lead to a selective excitation of the occurring bonding and antibonding chiral plasmonic modes.
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Citations
Cites
Classical Electrodynamics, 3rd ed .
Jackson, J. D., & Fox, R. F. (1999) · American Journal of Physics · doi:10.1119/1.19136 · Cited by 3,073
Cited by
Hentschel, M., Schäferling, M., Duan, X., Giessen, H., & Liu, N. (2017) · Science Advances · doi:10.1126/sciadv.1602735 · Cited by 850
Self-citationCatenary optics for achromatic generation of perfect optical angular momentum
Pu, M., Li, X., Ma, X., Wang, Y., Zhao, Z., Wang, C., Hu, C., Gao, P., Huang, C., Ren, H., et al. (2015) · Science Advances · doi:10.1126/sciadv.1500396 · Cited by 744
Electromagnetic chirality: from fundamentals to nontraditional chiroptical phenomena
Mun, J., Kim, M., Yang, Y., Badloe, T., Ni, J., Chen, Y., Qiu, C.-W., & Rho, J. (2020) · Light: Science & Applications · doi:10.1038/s41377-020-00367-8 · Cited by 573
A plasmonic nanorod that walks on DNA origami
Zhou, C., Duan, X., & Liu, N. (2015) · Nature Communications · doi:10.1038/ncomms9102 · Cited by 332
Topological Photonic Phase in Chiral Hyperbolic Metamaterials
Gao, W., Lawrence, M., Yang, B., Liu, F., Fang, F., Béri, B., Li, J., & Zhang, S. (2015) · Physical Review Letters · doi:10.1103/physrevlett.114.037402 · Cited by 314
Metadata
- Authors
- Yin, X., Schäferling, M., Metzger, B., & Giessen, H.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-11-27
- Volume
- 13
- Issue
- 12
- Pages
- 6238-6243
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2331487889
- Cited by
- 430
- References
- 1
- FWCI
- 11.69
- Type
- journal article
- Language
- en
- Open access
- closed
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