The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Pyrolysis of Cellulose under Ammonia Leads to Nitrogen-Doped Nanoporous Carbon Generated through Methane Formation
Abstract
Here, we present a simple one-step fabrication methodology for nitrogen-doped (N-doped) nanoporous carbon membranes via annealing cellulose filter paper under NH3. We found that nitrogen doping (up to 10.3 at %) occurs during cellulose pyrolysis under NH3 at as low as 550 °C. At 700 °C or above, N-doped carbon further reacts with NH3, resulting in a large surface area (up to 1973.3 m(2)/g). We discovered that the doped nitrogen, in fact, plays an important role in the reaction, leading to carbon gasification. CH4 was experimentally detected by mass spectrometry as a product in the reaction between N-doped carbon and NH3. When compared to conventional activated carbon (1533.6 m(2)/g), the N-doped nanoporous carbon (1326.5 m(2)/g) exhibits more than double the unit area capacitance (90 vs 41 mF/m(2)).
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Cites
Wang, H., Maiyalagan, T., & Wang, X. (2012) · ACS Catalysis · doi:10.1021/cs200652y · Cited by 3,618
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Self-citationWang, Q., Yan, J., & Fan, Z. (2016) · Energy & Environmental Science · doi:10.1039/c5ee03109e · Cited by 1,225
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Deng, J., Li, M., & Wang, Y. (2016) · Green Chemistry · doi:10.1039/c6gc01172a · Cited by 956
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Ayiania, M., Smith, M., Hensley, A. J. R., Scudiero, L., McEwen, J.-S., & Garcia-Perez, M. (2020) · Carbon · doi:10.1016/j.carbon.2020.02.065 · Cited by 906
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Metadata
- Authors
- Luo, W., Wang, B., Heron, C. G., Allen, M. J., Morre, J., Maier, C. S., Stickle, W. F., & Ji, X.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-04-01
- Volume
- 14
- Issue
- 4
- Pages
- 2225-2229
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2328392707
- Cited by
- 343
- References
- 1
- FWCI
- 12.01
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
