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Enhanced Third-Harmonic Generation in Silicon Nanoparticles Driven by Magnetic Response
Abstract
We observe enhanced third-harmonic generation from silicon nanodisks exhibiting both electric and magnetic dipolar resonances. Experimental characterization of the nonlinear optical response through third-harmonic microscopy and spectroscopy reveals that the third-harmonic generation is significantly enhanced in the vicinity of the magnetic dipole resonances. The field localization at the magnetic resonance results in two orders of magnitude enhancement of the harmonic intensity with respect to unstructured bulk silicon with the conversion efficiency limited only by the two-photon absorption in the substrate.
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Classical Electrodynamics, 3rd ed .
Jackson, J. D., & Fox, R. F. (1999) · American Journal of Physics · doi:10.1119/1.19136 · Cited by 3,073
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Krasnok, A., Tymchenko, M., & Alù, A. (2018) · Materials Today · doi:10.1016/j.mattod.2017.06.007 · Cited by 613
Nonlinear Metasurfaces Governed by Bound States in the Continuum
Koshelev, K., Tang, Y., Li, K., Choi, D.-Y., Li, G., & Kivshar, Y. (2019) · ACS Photonics · doi:10.1021/acsphotonics.9b00700 · Cited by 561
Self-citationNon-plasmonic nanoantennas for surface enhanced spectroscopies with ultra-low heat conversion
Caldarola, M., Albella, P., Cortés, E., Rahmani, M., Roschuk, T., Grinblat, G., Oulton, R. F., Bragas, A. V., & Maier, S. A. (2015) · Nature Communications · doi:10.1038/ncomms8915 · Cited by 520
All-dielectric nanophotonics: the quest for better materials and fabrication techniques
Baranov, D. G., Zuev, D. A., Lepeshov, S. I., Kotov, O. V., Krasnok, A. E., Evlyukhin, A. B., & Chichkov, B. N. (2017) · Optica · doi:10.1364/optica.4.000814 · Cited by 462
Metadata
- Authors
- Shcherbakov, M. R., Neshev, D. N., Hopkins, B., Shorokhov, A. S., Staude, I., Melik-Gaykazyan, E. V., Decker, M., Ezhov, A. A., Miroshnichenko, A. E., Brener, I., Fedyanin, A. A., & Kivshar, Y. S.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-10-21
- Volume
- 14
- Issue
- 11
- Pages
- 6488-6492
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2034687471
- Cited by
- 629
- References
- 1
- FWCI
- 28.14
- Type
- journal article
- Language
- en
- Open access
- closed
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- Shcherbakov, M. R., Neshev, D. N., Hopkins, B., Shorokhov, A. S., Staude, I., Melik-Gaykazyan, E. V., Decker, M., Ezhov, A. A., Miroshnichenko, A. E., Brener, I., Fedyanin, A. A., & Kivshar, Y. S. (2014). Enhanced Third-Harmonic Generation in Silicon Nanoparticles Driven by Magnetic Response. Nano Letters. https://doi.org/10.1021/nl503029j
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