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Integrated Perovskite/Bulk-Heterojunction toward Efficient Solar Cells

Liu, Yongsheng, Hong, Ziruo, Chen, Qi, Chang, Weihsuan, Zhou, Huanping, Song, Tze-Bin, Young, Eric, Yang, Yang (Michael), You, Jingbi, Li, Gang, Yang, Yang·2015·Nano Letters

Abstract

We successfully demonstrated an integrated perovskite/bulk-heterojunction (BHJ) photovoltaic device for efficient light harvesting and energy conversion. Our device efficiently integrated two photovoltaic layers, namely a perovskite film and organic BHJ film, into the device. The device structure is ITO/TiO2/perovskite/BHJ/MoO3/Ag. A wide bandgap small molecule DOR3T-TBDT was used as donor in the BHJ film, and a power conversion efficiency (PCE) of 14.3% was achieved in the integrated device with a high short circuit current density (JSC) of 21.2 mA cm(-2). The higher JSC as compared to that of the traditional perovskite/HTL (hole transporting layer) device (19.3 mA cm(-2)) indicates that the BHJ film absorbs light and contributes to the current density of the device. Our result further suggests that the HTL in traditional perovskite solar cell, even with good light absorption capability, cannot contribute to the overall device photocurrent, unless this HTL becomes a BHJ layer (by adding electron transporting material like PC71BM).

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Metadata

Authors
Liu, Y., Hong, Z., Chen, Q., Chang, W., Zhou, H., Song, T.-B., Young, E., Yang, Y. (., You, J., Li, G., & Yang, Y.
Venue
Nano Letters
Published
2014-12-18
Volume
15
Issue
1
Pages
662-668
ISSN
  • 1530-6984 (ISSN-L)
  • 1530-6992
OpenAlex
W2330552328
Cited by
160
References
1
FWCI
8.49
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: Integrated Perovskite/Bulk-Heterojunction toward Efficient Solar Cells. https://app.cochat.ai/papers/10.1021/nl504168q
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Liu, Y., Hong, Z., Chen, Q., Chang, W., Zhou, H., Song, T.-B., Young, E., Yang, Y. (., You, J., Li, G., & Yang, Y. (2015). Integrated Perovskite/Bulk-Heterojunction toward Efficient Solar Cells. Nano Letters. https://doi.org/10.1021/nl504168q

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