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Quantum Plasmonics: Optical Properties and Tunability of Metallic Nanorods
Abstract
The plasmon resonances in metallic nanorods are investigated using fully quantum mechanical time-dependent density functional theory. The computed optical absorption curves display well-defined longitudinal and transverse plasmon resonances whose energies depend on the aspect ratio of the rods, in excellent agreement with classical electromagnetic modeling. The field enhancements obtained from the quantum mechanical calculations, however, differ significantly from classical predictions for distances shorter than 0.5 nm from the nanoparticle surfaces. These deviations can be understood as arising from the nonlocal screening properties of the conduction electrons at the nanoparticle surface.
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Cites
Self-interaction correction to density-functional approximations for many-electron systems
Perdew, J. P., & Zunger, A. (1981) · Physical Review B · doi:10.1103/physrevb.23.5048 · Cited by 20,887
Cited by
Strong coupling between surface plasmon polaritons and emitters: a review
Törmä, P., & Barnes, W. L. (2015) · Reports on Progress in Physics · doi:10.1088/0034-4885/78/1/013901 · Cited by 1,644
Tame, M. S., McEnery, K. R., Özdemir, Ş. K., Lee, J., Maier, S. A., & Kim, M. S. (2013) · Nature Physics · doi:10.1038/nphys2615 · Cited by 1,573
Nanoplasmonics: Past, present, and glimpse into future
Stockman, M. I. (2011) · Optics Express · doi:10.1364/oe.19.022029 · Cited by 1,109
Quantum mechanical effects in plasmonic structures with subnanometre gaps
Zhu, W., Esteban, R., Borisov, A. G., Baumberg, J. J., Nordlander, P., Lezec, H. J., Aizpurua, J., & Crozier, K. B. (2016) · Nature Communications · doi:10.1038/ncomms11495 · Cited by 820
Self-citationBrown, L. V., Yang, X., Zhao, K., Zheng, B. Y., Nordlander, P., & Halas, N. J. (2015) · Nano Letters · doi:10.1021/nl504455s · Cited by 266
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Metadata
- Authors
- Zuloaga, J., Prodan, E., & Nordlander, P.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-08-10
- Volume
- 4
- Issue
- 9
- Pages
- 5269-5276
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W1979692431
- Cited by
- 241
- References
- 1
- FWCI
- 14.02
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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