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Pillaring Chemically Exfoliated Graphene Oxide with Carbon Nanotubes for Photocatalytic Degradation of Dyes under Visible Light Irradiation
Abstract
Graphene oxide (GO) and reduced graphene oxide (RGO) platelets were pillared with carbon nanotubes (CNTs) by using the chemical vapor deposition (CVD) method with acetonitrile as the carbon source and nickel nanoparticles as the catalyst, aimed to prepare graphene-based materials with a high surface area and a good electrical conductivity. Characterization data showed that the composite materials with RGO layers pillared by CNTs formed a robust three-dimensional (3D) porous structure of specific surfaces as high as 352 m(2)/g. The amount and length of the CNT pillars connecting the RGO layers were controlled by changing the amount of the nickel metal catalyst and the time of CVD. The CNT-pillared RGO composite materials exhibited an excellent visible light photocatalytic performance in degrading dye Rhodamine B because of the unique porous structure and the exceptional electron transfer property of graphene. Such CNT-RGO composites represent a new family of innovative carbon materials for visible-light-activated photocatalysis.
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Cites
Superior Thermal Conductivity of Single-Layer Graphene
Balandin, A. A., Ghosh, S., Bao, W., Calizo, I., Teweldebrhan, D., Miao, F., & Lau, C. N. (2008) · Nano Letters · doi:10.1021/nl0731872 · Cited by 13,823
Zhao, D., Chen, C., Wang, Y., Ma, W., Zhao, J., Rajh, T., & Zang, L. (2008) · Environmental Science & Technology · doi:10.1021/es071770e · Cited by 194
Cited by
Graphene-based semiconductor photocatalysts
Xiang, Q., Yu, J., & Jaroniec, M. (2012) · Chem. Soc. Rev. · doi:10.1039/c1cs15172j · Cited by 2,730
Metal-Free Catalysts for Oxygen Reduction Reaction
Dai, L., Xue, Y., Qu, L., Choi, H.-J., & Baek, J.-B. (2015) · Chemical Reviews · doi:10.1021/cr5003563 · Cited by 2,380
Georgakilas, V., Perman, J. A., Tucek, J., & Zboril, R. (2015) · Chemical Reviews · doi:10.1021/cr500304f · Cited by 2,147
Hydrothermal Synthesis of Graphene-TiO2 Nanotube Composites with Enhanced Photocatalytic Activity
Perera, S. D., Mariano, R. G., Vu, K., Nour, N., Seitz, O., Chabal, Y., & Balkus, K. J. (2012) · ACS Catalysis · doi:10.1021/cs200621c · Cited by 963
Reduced Graphene Oxide for Catalytic Oxidation of Aqueous Organic Pollutants
Sun, H., Liu, S., Zhou, G., Ang, H. M., Tadé, M. O., & Wang, S. (2012) · ACS Applied Materials & Interfaces · doi:10.1021/am301372d · Cited by 722
Metadata
- Authors
- Zhang, L. L., Xiong, Z., & Zhao, X. S.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-10-28
- Volume
- 4
- Issue
- 11
- Pages
- 7030-7036
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W1988303224
- Cited by
- 265
- References
- 2
- FWCI
- 10.08
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhang, L. L., Xiong, Z., & Zhao, X. S. (2010). Pillaring Chemically Exfoliated Graphene Oxide with Carbon Nanotubes for Photocatalytic Degradation of Dyes under Visible Light Irradiation. ACS Nano. https://doi.org/10.1021/nn102308r
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