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Raman 2D-Band Splitting in Graphene: Theory and Experiment
Open accessAbstract
We present a systematic experimental and theoretical study of the two-phonon (2D) Raman scattering in graphene under uniaxial tension. The external perturbation unveils that the 2D mode excited with 785 nm has a complex line-shape mainly due to the contribution of two distinct double resonance scattering processes (inner and outer) in the Raman signal. The splitting depends on the direction of the applied strain and the polarization of the incident light. The results give new insight into the nature of the 2D band and have significant implications for the use of graphene as reinforcement in composites since the 2D mode is crucial to assess how effectively graphene uptakes an applied stress or strain.
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Citations
Cites
Graphene: Status and Prospects
Geim, A. K. (2009) · Science · doi:10.1126/science.1158877 · Cited by 13,942
Energy gaps and a zero-field quantum Hall effect in graphene by strain engineering
Guinea, F., Katsnelson, M. I., & Geim, A. K. (2010) · Nature Physics · doi:10.1038/nphys1420 · Cited by 1,913
Cited by
Mechanical properties of graphene and graphene-based nanocomposites
Papageorgiou, D. G., Kinloch, I. A., & Young, R. J. (2017) · Progress in Materials Science · doi:10.1016/j.pmatsci.2017.07.004 · Cited by 2,579
The mechanics of graphene nanocomposites: A review
Young, R. J., Kinloch, I. A., Gong, L., & Novoselov, K. S. (2012) · Composites Science and Technology · doi:10.1016/j.compscitech.2012.05.005 · Cited by 1,294
Self-citationRaman spectroscopy of carbon materials and their composites: Graphene, nanotubes and fibres
Li, Z., Deng, L., Kinloch, I. A., & Young, R. J. (2023) · Progress in Materials Science · doi:10.1016/j.pmatsci.2023.101089 · Cited by 1,117
Fast and fully-scalable synthesis of reduced graphene oxide
Abdolhosseinzadeh, S., Asgharzadeh, H., & Seop Kim, H. (2015) · Scientific Reports · doi:10.1038/srep10160 · Cited by 667
Zhang, F., Feng, Y., Qin, M., Gao, L., Li, Z., Zhao, F., Zhang, Z., Lv, F., & Feng, W. (2019) · Advanced Functional Materials · doi:10.1002/adfm.201901383 · Cited by 308
Metadata
- Authors
- Frank, O., Mohr, M., Maultzsch, J., Thomsen, C., Riaz, I., Jalil, R., Novoselov, K. S., Tsoukleri, G., Parthenios, J., Papagelis, K., Kavan, L., & Galiotis, C.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-02-14
- Volume
- 5
- Issue
- 3
- Pages
- 2231-2239
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2012071323
- Cited by
- 319
- References
- 2
- FWCI
- 11.15
- Type
- journal article
- Language
- en
- Open access
- green
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- Frank, O., Mohr, M., Maultzsch, J., Thomsen, C., Riaz, I., Jalil, R., Novoselov, K. S., Tsoukleri, G., Parthenios, J., Papagelis, K., Kavan, L., & Galiotis, C. (2011). Raman 2D-Band Splitting in Graphene: Theory and Experiment. ACS Nano. https://doi.org/10.1021/nn103493g
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