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Graphene Oxide Enwrapped Ag/AgX (X = Br, Cl) Nanocomposite as a Highly Efficient Visible-Light Plasmonic Photocatalyst

Zhu, Mingshan, Chen, Penglei, Liu, Minghua·2011·ACS Nano

Abstract

In this paper, we have reported that well-defined graphene oxide (GO) enwrapped Ag/AgX (X = Br, Cl) nanocomposites, which are composed of Ag/AgX nanoparticles and gauze-like GO nanosheets, could be facilely fabricated via a water/oil system. We have shown that thus-synthesized GO-based hybrid nanocomposites could be used as a stable plasmonic photocatalyst for the photodegradation of methyl orange (MO) pollutant under visible-light irradiation. Compared with the corresponding bare Ag/AgX nanospecies, the GO-involved nanocomposites (Ag/AgX/GO) display distinctly enhanced photocatalytic activities. The hybridization of Ag/AgX with GO nanosheets causes the nice adsorptive capacity of Ag/AgX/GO to MO molecules, the smaller size of the Ag/AgX nanoparticles in Ag/AgX/GO, the facilitated charge transfer, and the suppressed recombination of electron-hole pairs in Ag/AgX/GO. It is suggested that these multifactors, resulting from the hybridization of GO, contribute to the enhanced photocatalytic performance observed from Ag/AgX/GO. The investigation likely opens up new possibilities for the development of original yet highly efficient and stable GO-based plasmonic photocatalysts that utilize visible light as an energy source.

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Metadata

Authors
Zhu, M., Chen, P., & Liu, M.
Venue
ACS Nano
Published
2011-05-06
Volume
5
Issue
6
Pages
4529-4536
ISSN
  • 1936-0851 (ISSN-L)
  • 1936-086X
OpenAlex
W2325830109
Cited by
696
References
5
FWCI
31.13
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: Graphene Oxide Enwrapped Ag/AgX (X = Br, Cl) Nanocomposite as a Highly Efficient Visible-Light Plasmonic Photocatalyst. https://app.cochat.ai/papers/10.1021/nn200088x
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Zhu, M., Chen, P., & Liu, M. (2011). Graphene Oxide Enwrapped Ag/AgX (X = Br, Cl) Nanocomposite as a Highly Efficient Visible-Light Plasmonic Photocatalyst. ACS Nano. https://doi.org/10.1021/nn200088x

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