The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Catalytic Hydrolysis of Ammonia Borane via Cobalt Palladium Nanoparticles
Abstract
Monodisperse 8 nm CoPd nanoparticles (NPs) with controlled compositions were synthesized by the reduction of cobalt acetylacetonate and palladium bromide in the presence of oleylamine and trioctylphosphine. These NPs were active catalysts for hydrogen generation from the hydrolysis of ammonia borane (AB), and their activities were composition dependent. Among the 8 nm CoPd catalysts tested for the hydrolysis of AB, the Co(35)Pd(65) NPs exhibited the highest catalytic activity and durability. Their hydrolysis completion time and activation energy were 5.5 min and 27.5 kJ mol(-1), respectively, which were comparable to the best Pt-based catalyst reported. The catalytic performance of the CoPd/C could be further enhanced by a preannealing treatment at 300 °C under air for 15 h with the hydrolysis completion time reduced to 3.5 min. This high catalytic performance of Co(35)Pd(65) NP catalyst makes it an exciting alternative in pursuit of practical implementation of AB as a hydrogen storage material for fuel cell applications.
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Cites
Chemistry and Properties of Nanocrystals of Different Shapes
Burda, C., Chen, X., Narayanan, R., & El-Sayed, M. A. (2005) · Chemical Reviews · doi:10.1021/cr030063a · Cited by 7,230
Computational high-throughput screening of electrocatalytic materials for hydrogen evolution
Greeley, J., Jaramillo, T. F., Bonde, J., Chorkendorff, I., & Nørskov, J. K. (2006) · Nature Materials · doi:10.1038/nmat1752 · Cited by 4,097
B–N compounds for chemical hydrogenstorage
Hamilton, C. W., Baker, R. T., Staubitz, A., & Manners, I. (2009) · Chem. Soc. Rev. · doi:10.1039/b800312m · Cited by 1,087
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Synergistic Catalysis over Bimetallic Alloy Nanoparticles
Singh, A. K., & Xu, Q. (2013) · ChemCatChem · doi:10.1002/cctc.201200591 · Cited by 698
Organic Phase Syntheses of Magnetic Nanoparticles and Their Applications
Wu, L., Mendoza-Garcia, A., Li, Q., & Sun, S. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00687 · Cited by 601
Self-citationSynthesis and catalytic properties of bimetallic nanomaterials with various architectures
Liu, X., Wang, D., & Li, Y. (2012) · Nano Today · doi:10.1016/j.nantod.2012.08.003 · Cited by 538
Microwave-assisted optimization of platinum-nickel nanoalloys for catalytic water treatment
Ma, H., Wang, H., & Na, C. (2015) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2014.07.062 · Cited by 76
A review on hydrogen production from ammonia borane: Experimental and theoretical studies
Huo, J., Zhang, K., Wei, H., Fu, L., Zhao, C., He, C., & Hu, X. (2023) · Chinese Chemical Letters · doi:10.1016/j.cclet.2023.108280 · Cited by 53
Metadata
- Authors
- Sun, D., Mazumder, V., Metin, Ö., & Sun, S.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2011-07-21
- Volume
- 5
- Issue
- 8
- Pages
- 6458-6464
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2084653571
- Cited by
- 273
- References
- 3
- FWCI
- 12.39
- Type
- journal article
- Language
- en
- Open access
- closed
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