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Building Robust Architectures of Carbon and Metal Oxide Nanocrystals toward High-Performance Anodes for Lithium-Ion Batteries
Abstract
Design and fabrication of effective electrode structure is essential but is still a challenge for current lithium-ion battery technology. Herein we report the design and fabrication of a class of high-performance robust nanocomposites based on iron oxide spheres and carbon nanotubes (CNTs). An efficient aerosol spray process combined with vacuum filtration was used to synthesize such composite architecture, where oxide nanocrystals were assembled into a continuous carbon skeleton and entangled in porous CNT networks. This material architecture offers many critical features that are required for high-performance anodes, including efficient ion transport, high conductivity, and structure durability, therefore enabling an electrode with outstanding lithium storage performance. For example, such an electrode with a thickness of ∼35 μm could deliver a specific capacity of 994 mA h g(-1) (based on total electrode weight) and high recharging rates. This effective strategy can be extended to construct many other composite electrodes for high-performance lithium-ion batteries.
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Cites
Lithium Batteries: Status, Prospects and Future
Scrosati, B., & Garche, J. (2010) · Journal of Power Sources · doi:10.1016/j.jpowsour.2009.11.048 · Cited by 5,153
Cited by
Luo, J., Liu, J., Zeng, Z., Ng, C. F., Ma, L., Zhang, H., Lin, J., Shen, Z., & Fan, H. J. (2013) · Nano Letters · doi:10.1021/nl403461n · Cited by 773
Peng, S., Li, L., Han, X., Sun, W., Srinivasan, M., Mhaisalkar, S. G., Cheng, F., Yan, Q., Chen, J., & Ramakrishna, S. (2014) · Angewandte Chemie International Edition · doi:10.1002/anie.201408876 · Cited by 428
Silicon oxycarbide glass-graphene composite paper electrode for long-cycle lithium-ion batteries
David, L., Bhandavat, R., Barrera, U., & Singh, G. (2016) · Nature Communications · doi:10.1038/ncomms10998 · Cited by 389
Li, L., Raji, A. O., & Tour, J. M. (2013) · Advanced Materials · doi:10.1002/adma.201302915 · Cited by 381
Peng, S., Li, L., Han, X., Sun, W., Srinivasan, M., Mhaisalkar, S. G., Cheng, F., Yan, Q., Chen, J., & Ramakrishna, S. (2014) · Angewandte Chemie · doi:10.1002/ange.201408876 · Cited by 209
Metadata
- Authors
- Jia, X., Chen, Z., Cui, X., Peng, Y., Wang, X., Wang, G., Wei, F., & Lu, Y.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-11-01
- Volume
- 6
- Issue
- 11
- Pages
- 9911-9919
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2051587557
- Cited by
- 174
- References
- 1
- FWCI
- 17.50
- Type
- journal article
- Language
- en
- Open access
- closed
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- Jia, X., Chen, Z., Cui, X., Peng, Y., Wang, X., Wang, G., Wei, F., & Lu, Y. (2012). Building Robust Architectures of Carbon and Metal Oxide Nanocrystals toward High-Performance Anodes for Lithium-Ion Batteries. ACS Nano. https://doi.org/10.1021/nn303478e
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