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Organic Solvent-Based Graphene Oxide Liquid Crystals: A Facile Route toward the Next Generation of Self-Assembled Layer-by-Layer Multifunctional 3D Architectures
Open accessAbstract
We introduce soft self-assembly of ultralarge liquid crystalline (LC) graphene oxide (GO) sheets in a wide range of organic solvents overcoming the practical limitations imposed on LC GO processing in water. This expands the number of known solvents which can support amphiphilic self-assembly to ethanol, acetone, tetrahydrofuran, N-dimethylformamide, N-cyclohexyl-2-pyrrolidone, and a number of other organic solvents, many of which were not known to afford solvophobic self-assembly prior to this report. The LC behavior of the as-prepared GO sheets in organic solvents has enabled us to disperse and organize substantial amounts of aggregate-free single-walled carbon nanotubes (SWNTs, up to 10 wt %) without compromise in LC properties. The as-prepared LC GO-SWNT dispersions were employed to achieve self-assembled layer-by-layer multifunctional 3D hybrid architectures comprising SWNTs and GO with unrivalled superior mechanical properties (Young's modulus in excess of 50 GPa and tensile strength of more than 500 MPa).
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Citations
Cited by
Graphene-polymer nanocomposites for structural and functional applications
Hu, K., Kulkarni, D. D., Choi, I., & Tsukruk, V. V. (2014) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2014.03.001 · Cited by 1,085
Brisebois, P. P., & Siaj, M. (2020) · Journal of Materials Chemistry C · doi:10.1039/c9tc03251g · Cited by 445
Lian, G., Tuan, C.-C., Li, L., Jiao, S., Wang, Q., Moon, K.-S., Cui, D., & Wong, C.-P. (2016) · Chemistry of Materials · doi:10.1021/acs.chemmater.6b01595 · Cited by 382
Rhazouani, A., Gamrani, H., El Achaby, M., Aziz, K., Gebrati, L., Uddin, M. S., & AZIZ, F. (2021) · BioMed Research International · doi:10.1155/2021/5518999 · Cited by 221
Metadata
- Authors
- Jalili, R., Aboutalebi, S. H., Esrafilzadeh, D., Konstantinov, K., Moulton, S. E., Razal, J. M., & Wallace, G. G.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-04-22
- Volume
- 7
- Issue
- 5
- Pages
- 3981-3990
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W1514234853
- Cited by
- 244
- References
- 0
- FWCI
- 11.99
- Type
- journal article
- Language
- en
- Open access
- green
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- Jalili, R., Aboutalebi, S. H., Esrafilzadeh, D., Konstantinov, K., Moulton, S. E., Razal, J. M., & Wallace, G. G. (2013). Organic Solvent-Based Graphene Oxide Liquid Crystals: A Facile Route toward the Next Generation of Self-Assembled Layer-by-Layer Multifunctional 3D Architectures. ACS Nano. https://doi.org/10.1021/nn305906z
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