The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Ultrafast Carrier Thermalization and Cooling Dynamics in Few-Layer MoS2
Abstract
Femtosecond optical pump-probe spectroscopy with 10 fs visible pulses is employed to elucidate the ultrafast carrier dynamics of few-layer MoS2. A nonthermal carrier distribution is observed immediately following the photoexcitation of the A and B excitonic transitions by the ultrashort, broadband laser pulse. Carrier thermalization occurs within 20 fs and proceeds via both carrier-carrier and carrier-phonon scattering, as evidenced by the observed dependence of the thermalization time on the carrier density and the sample temperature. The n(-0.37 ± 0.03) scaling of the thermalization time with carrier density suggests that equilibration of the nonthermal carrier distribution occurs via non-Markovian quantum kinetics. Subsequent cooling of the hot Fermi-Dirac carrier distribution occurs on the ∼ 0.6 ps time scale via carrier-phonon scattering. Temperature- and fluence-dependence studies reveal the involvement of hot phonons in the carrier cooling process. Nonadiabatic ab initio molecular dynamics simulations, which predict carrier-carrier and carrier-phonon scattering time scales of 40 fs and 0.5 ps, respectively, lend support to the assignment of the observed carrier dynamics.
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The electronic properties of graphene
Castro Neto, A. H., Guinea, F., Peres, N. M. R., Novoselov, K. S., & Geim, A. K. (2009) · Reviews of Modern Physics · doi:10.1103/revmodphys.81.109 · Cited by 24,803
Electronics and optoelectronics of two-dimensional transition metal dichalcogenides
Wang, Q. H., Kalantar-Zadeh, K., Kis, A., Coleman, J. N., & Strano, M. S. (2012) · Nature Nanotechnology · doi:10.1038/nnano.2012.193 · Cited by 16,374
The chemistry of two-dimensional layered transition metal dichalcogenide nanosheets
Chhowalla, M., Shin, H. S., Eda, G., Li, L.-J., Loh, K. P., & Zhang, H. (2013) · Nature Chemistry · doi:10.1038/nchem.1589 · Cited by 10,034
Cited by
Photonics of time-varying media
Galiffi, E., Tirole, R., Yin, S., Li, H., Vezzoli, S., Huidobro, P. A., Silveirinha, M. G., Sapienza, R., Alù, A., & Pendry, J. B. (2022) · Advanced Photonics · doi:10.1117/1.ap.4.1.014002 · Cited by 591
Zheng, Q., Chu, W., Zhao, C., Zhang, L., Guo, H., Wang, Y., Jiang, X., & Zhao, J. (2019) · WIREs Computational Molecular Science · doi:10.1002/wcms.1411 · Cited by 452
Metadata
- Authors
- Nie, Z., Long, R., Sun, L., Huang, C.-C., Zhang, J., Xiong, Q., Hewak, D. W., Shen, Z., Prezhdo, O. V., & Loh, Z.-H.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-10-02
- Volume
- 8
- Issue
- 10
- Pages
- 10931-10940
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2127527950
- Cited by
- 310
- References
- 3
- FWCI
- 8.93
- Type
- journal article
- Language
- en
- Open access
- closed
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- Nie, Z., Long, R., Sun, L., Huang, C.-C., Zhang, J., Xiong, Q., Hewak, D. W., Shen, Z., Prezhdo, O. V., & Loh, Z.-H. (2014). Ultrafast Carrier Thermalization and Cooling Dynamics in Few-Layer MoS2. ACS Nano. https://doi.org/10.1021/nn504760x
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