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Photothermal-Responsive Single-Walled Carbon Nanotube-Based Ultrathin Membranes for On/Off Switchable Separation of Oil-in-Water Nanoemulsions
Abstract
Oil-contaminated wastewater threatens our environment and health, especially that stabilized by surfactants. Conventional separation protocols become invalid for those surfactant-stabilized nanoemulsions due to their nanometer-sized droplets and extremely high stability. In this paper, photothermal-responsive ultrathin Au nanorods/poly(N-isopropylacrylamide-co-acrylamide) cohybrid single-walled carbon nanotube (SWCNT) nanoporous membranes are constructed. Such membranes are capable of separating oil-in-water nanoemulsions with a maximum flux up to 35 890 m(2)·h(-1)·bar(-1) because they feature hydrophilicity, underwater oleophobicity, and nanometer pore sizes. It is remarkable that the permeation flux can be simply modulated by light illumination during the process of separation, due to the incorporation of thermal-responsive copolymers and Au nanorods. Meanwhile, it shows ultrahigh separation efficiency (>99.99%) and desired antifouling and recyclability properties. We anticipate that our ultrathin photothermal-responsive SWCNT-based membranes provide potential for the generation of point-of-use water treatment devices.
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Cites
Mussel-inspired surface chemistry for multifunctional coatings
Lee, H., Dellatore, S. M., Miller, W. M., & Messersmith, P. B. (2007) · Science · doi:10.1126/science.1147241 · Cited by 10,965
Cited by
Ge, J., Zong, D., Jin, Q., Yu, J., & Ding, B. (2018) · Advanced Functional Materials · doi:10.1002/adfm.201705051 · Cited by 677
Carbon‐Based Photothermal Actuators
Han, B., Zhang, Y., Chen, Q., & Sun, H. (2018) · Advanced Functional Materials · doi:10.1002/adfm.201802235 · Cited by 522
Shi, H., He, Y., Pan, Y., Di, H., Zeng, G., Zhang, L., & Zhang, C. (2016) · Journal of Membrane Science · doi:10.1016/j.memsci.2016.01.053 · Cited by 485
Barclay, T. G., Hegab, H. M., Clarke, S. R., & Ginic‐Markovic, M. (2017) · Advanced Materials Interfaces · doi:10.1002/admi.201601192 · Cited by 384
Design and fabrication of superwetting fiber-based membranes for oil/water separation applications
Yue, X., Li, Z., Zhang, T., Yang, D., & Qiu, F. (2019) · Chemical Engineering Journal · doi:10.1016/j.cej.2019.01.149 · Cited by 384
Metadata
- Authors
- Hu, L., Gao, S., Ding, X., Wang, D., Jiang, J., Jin, J., & Jiang, L.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-04-27
- Volume
- 9
- Issue
- 5
- Pages
- 4835-4842
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W1970196150
- Cited by
- 284
- References
- 1
- FWCI
- 20.34
- Type
- journal article
- Language
- en
- Open access
- closed
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- Hu, L., Gao, S., Ding, X., Wang, D., Jiang, J., Jin, J., & Jiang, L. (2015). Photothermal-Responsive Single-Walled Carbon Nanotube-Based Ultrathin Membranes for On/Off Switchable Separation of Oil-in-Water Nanoemulsions. ACS Nano. https://doi.org/10.1021/nn5062854
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