The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Permselective Graphene Oxide Membrane for Highly Stable and Anti-Self-Discharge Lithium–Sulfur Batteries
Open accessAbstract
Lithium-sulfur batteries hold great promise for serving as next generation high energy density batteries. However, the shuttle of polysulfide induces rapid capacity degradation and poor cycling stability of lithium-sulfur cells. Herein, we proposed a unique lithium-sulfur battery configuration with an ultrathin graphene oxide (GO) membrane for high stability. The oxygen electronegative atoms modified GO into a polar plane, and the carboxyl groups acted as ion-hopping sites of positively charged species (Li(+)) and rejected the transportation of negatively charged species (Sn(2-)) due to the electrostatic interactions. Such electrostatic repulsion and physical inhibition largely decreased the transference of polysulfides across the GO membrane in the lithium-sulfur system. Consequently, the GO membrane with highly tunable functionalization properties, high mechanical strength, low electric conductivity, and facile fabrication procedure is an effective permselective separator system in lithium-sulfur batteries. By the incorporation of a permselective GO membrane, the cyclic capacity decay rate is also reduced from 0.49 to 0.23%/cycle. As the GO membrane blocks the diffusion of polysulfides through the membrane, it is also with advantages of anti-self-discharge properties.
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Cites
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Cited by
Smith, A. T., LaChance, A. M., Zeng, S., Liu, B., & Sun, L. (2019) · Nano Materials Science · doi:10.1016/j.nanoms.2019.02.004 · Cited by 1,643
Graphene for batteries, supercapacitors and beyond
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Graphene Properties, Synthesis and Applications: A Review
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Rational Design of Nanostructured Functional Interlayer/Separator for Advanced Li–S Batteries
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Graphene oxide: An emerging electromaterial for energy storage and conversion
Tian, Y., Yu, Z., Cao, L., Zhang, X. L., Sun, C., & Wang, D.-W. (2021) · Journal of Energy Chemistry · doi:10.1016/j.jechem.2020.07.006 · Cited by 240
Metadata
- Authors
- Huang, J.-Q., Zhuang, T.-Z., Zhang, Q., Peng, H.-J., Chen, C.-M., & Wei, F.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-02-18
- Volume
- 9
- Issue
- 3
- Pages
- 3002-3011
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2048782510
- Cited by
- 809
- References
- 1
- FWCI
- 45.55
- Type
- journal article
- Language
- en
- Open access
- hybrid
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