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Determination of the Exciton Binding Energy in CdSe Quantum Dots
Open accessAbstract
The exciton binding energy (EBE) in CdSe quantum dots (QDs) has been determined using X-ray spectroscopy. Using X-ray absorption and photoemission spectroscopy, the conduction band (CB) and valence band (VB) edge shifts as a function of particle size have been determined and combined to obtain the true band gap of the QDs (i.e., without an exciton). These values can be compared to the excitonic gap obtained using optical spectroscopy to determine the EBE. The experimental EBE results are compared with theoretical calculations on the EBE and show excellent agreement.
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Cites
Perspectives on the Physical Chemistry of Semiconductor Nanocrystals
Alivisatos, A. P. (1996) · The Journal of Physical Chemistry · doi:10.1021/jp9535506 · Cited by 3,595
Cited by
Size-Dependent Valence and Conduction Band-Edge Energies of Semiconductor Nanocrystals
Jasieniak, J., Califano, M., & Watkins, S. E. (2011) · ACS Nano · doi:10.1021/nn201681s · Cited by 699
The Evolution of Quantum Confinement in CsPbBr3 Perovskite Nanocrystals
Butkus, J., Vashishtha, P., Chen, K., Gallaher, J. K., Prasad, S. K. K., Metin, D. Z., Laufersky, G., Gaston, N., Halpert, J. E., & Hodgkiss, J. M. (2017) · Chemistry of Materials · doi:10.1021/acs.chemmater.7b00478 · Cited by 362
Metadata
- Authors
- Meulenberg, R. W., Lee, J. R. I., Wolcott, A., Zhang, J. Z., Terminello, L. J., & van Buuren, T.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2009-02-03
- Volume
- 3
- Issue
- 2
- Pages
- 325-330
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2103933439
- Cited by
- 180
- References
- 1
- FWCI
- 3.99
- Type
- journal article
- Language
- en
- Open access
- green
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- Meulenberg, R. W., Lee, J. R. I., Wolcott, A., Zhang, J. Z., Terminello, L. J., & van Buuren, T. (2009). Determination of the Exciton Binding Energy in CdSe Quantum Dots. ACS Nano. https://doi.org/10.1021/nn8006916
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