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Estimate of global atmospheric organic aerosol from oxidation of biogenic hydrocarbons
Open accessAbstract
The results from a series of outdoor chamber experiments establishing the atmospheric aerosol‐forming potential of fourteen terpenoid hydrocarbons have been used to estimate the annual amount of secondary organic aerosol formed globally from compounds emitted by vegetation. Hydroxyl radical, ozone, and nitrate radical oxidation each contribute to aerosol formation in full‐photooxidation experiments; because oxidation by nitrate radical under ambient, remote conditions is likely to be negligible, parameters describing aerosol formation from hydroxyl radical and ozone reaction only are developed. Chamber results, temporally and spatially resolved, compound‐specific estimates of biogenic hydrocarbon emissions, and hydroxyl radical and ozone fields are combined to lead to an estimate for atmospheric secondary organic aerosol formed annually from biogenic precursors of 18.5 Tg, a number smaller than the previously published estimate of 30–270 Tg [Andreae and Crutzen, 1997].
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Cited by
Organic aerosol and global climate modelling: a review
Kanakidou, M., Seinfeld, J. H., Pandis, S. N., Barnes, I., Dentener, F. J., Facchini, M. C., Van Dingenen, R., Ervens, B., Nenes, A., Nielsen, C. J., et al. (2005) · Atmospheric Chemistry and Physics · doi:10.5194/acp-5-1053-2005 · Cited by 3,244
Self-citationGlobal distribution and climate forcing of carbonaceous aerosols
Chung, S. H., & Seinfeld, J. H. (2002) · Journal of Geophysical Research: Atmospheres · doi:10.1029/2001jd001397 · Cited by 697
Self-citationNighttime radical observations and chemistry
Brown, S. S., & Stutz, J. (2012) · Chemical Society Reviews · doi:10.1039/c2cs35181a · Cited by 637
Chemistry and the Linkages between Air Quality and Climate Change
von Schneidemesser, E., Monks, P. S., Allan, J. D., Bruhwiler, L., Forster, P., Fowler, D., Lauer, A., Morgan, W. T., Paasonen, P., Righi, M., et al. (2015) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00089 · Cited by 522
Kleindienst, T. E., Jaoui, M., Lewandowski, M., Offenberg, J. H., Lewis, C. W., Bhave, P. V., & Edney, E. O. (2007) · Atmospheric Environment · doi:10.1016/j.atmosenv.2007.06.045 · Cited by 502
Metadata
- Authors
- Griffin, R. J., Cocker, D. R., Seinfeld, J. H., & Dabdub, D.
- Venue
- Geophysical Research Letters
- Publisher
- American Geophysical Union (AGU)
- Published
- 1999-09
- Volume
- 26
- Issue
- 17
- Pages
- 2721-2724
- ISSN
- 0094-8276 (ISSN-L)
- 1944-8007
- OpenAlex
- W2126894581
- Cited by
- 367
- References
- 0
- FWCI
- 6.75
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Griffin, R. J., Cocker, D. R., Seinfeld, J. H., & Dabdub, D. (1999). Estimate of global atmospheric organic aerosol from oxidation of biogenic hydrocarbons. Geophysical Research Letters. https://doi.org/10.1029/1999gl900476
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.