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Impact of new laboratory studies of N2O5 hydrolysis on global model budgets of tropospheric nitrogen oxides, ozone, and OH
Open accessAbstract
We investigate the impact of new laboratory studies of N 2 O 5 hydrolysis in aerosols on global model simulations of tropospheric chemistry. We use data from these new studies to parameterize the reaction probability (γ N2O5) in the GEOS‐CHEM global model as a function of local aerosol composition, temperature, and relative humidity. We find a much lower global mean γ N2O5 (0.02) than commonly assumed in models (0.1). Relative to a model simulation assuming a uniform γ N2O5 = 0.1, we find increases in mass‐averaged tropospheric NO x, O 3, and OH concentrations of 7%, 4%, and 8% respectively. The increases in NO x and O 3 concentrations bring the GEOS‐CHEM simulation in better agreement with climatological observations.
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Cites
Evidence for Substantial Variations of Atmospheric Hydroxyl Radicals in the Past Two Decades
Prinn, R. G., Huang, J., Weiss, R. F., Cunnold, D. M., Fraser, P. J., Simmonds, P. G., McCulloch, A., Harth, C., Salameh, P., O'Doherty, S., et al. (2001) · Science · doi:10.1126/science.1058673 · Cited by 695
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Li, K., Jacob, D. J., Liao, H., Shen, L., Zhang, Q., & Bates, K. H. (2019) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.1812168116 · Cited by 1,804
Self-citationFormation of Urban Fine Particulate Matter
Zhang, R., Wang, G., Guo, S., Zamora, M. L., Ying, Q., Lin, Y., Wang, W., Hu, M., & Wang, Y. (2015) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00067 · Cited by 1,426
Development cycle 2 of the Modular Earth Submodel System (MESSy2)
Jöckel, P., Kerkweg, A., Pozzer, A., Sander, R., Tost, H., Riede, H., Baumgaertner, A., Gromov, S., & Kern, B. (2010) · Geoscientific Model Development · doi:10.5194/gmd-3-717-2010 · Cited by 551
Nighttime radical observations and chemistry
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Yu, F., & Luo, G. (2009) · Atmospheric Chemistry and Physics · doi:10.5194/acp-9-7691-2009 · Cited by 448
Metadata
- Authors
- Evans, M. J., & Jacob, D. J.
- Venue
- Geophysical Research Letters
- Publisher
- American Geophysical Union (AGU)
- Published
- 2005-05
- Volume
- 32
- Issue
- 9
- ISSN
- 0094-8276 (ISSN-L)
- 1944-8007
- OpenAlex
- W2097372672
- Cited by
- 345
- References
- 1
- FWCI
- 9.80
- Type
- journal article
- Language
- en
- Open access
- green
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- Evans, M. J., & Jacob, D. J. (2005). Impact of new laboratory studies of N2O5 hydrolysis on global model budgets of tropospheric nitrogen oxides, ozone, and OH. Geophysical Research Letters. https://doi.org/10.1029/2005gl022469
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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