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Evolution of mixing state of black carbon particles: Aircraft measurements over the western Pacific in March 2004
Open accessAbstract
We report the evolution of the mixing state of black carbon (BC) particles in urban plumes measured by an airborne single particle soot photometer. The aircraft observations were conducted over the ocean near the coast of Japan in March 2004. The number fraction of coated BC particles with a core diameter of 180 nm increased from 0.35 to 0.63 within 12 hours (h), namely 2.3% h−1, after being emitted from the Nagoya urban area in Japan. BC particles with a core diameter of 250 nm increased at the slower rate of 1.0% h−1. The increase in coated BC particles was associated with increases in non‐sea salt sulfate and water‐soluble organic carbon by a factor of approximately two, indicating that these compounds contributed to the coating on the BC particles. These results give direct evidence that BC particles become internally mixed on a time scale of 12 h in urban plumes.
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Cited by
Bounding the role of black carbon in the climate system: A scientific assessment
Bond, T. C., Doherty, S. J., Fahey, D. W., Forster, P. M., Berntsen, T., DeAngelo, B. J., Flanner, M. G., Ghan, S., Kärcher, B., Koch, D., et al. (2013) · Journal of Geophysical Research: Atmospheres · doi:10.1002/jgrd.50171 · Cited by 6,385
Self-citationPöschl, U., & Shiraiwa, M. (2015) · Chemical Reviews · doi:10.1021/cr500487s · Cited by 657
Aerosol Mixing State: Measurements, Modeling, and Impacts
Riemer, N., Ault, A. P., West, M., Craig, R. L., & Curtis, J. H. (2019) · Reviews of Geophysics · doi:10.1029/2018rg000615 · Cited by 459
Wang, X., Heald, C. L., Ridley, D. A., Schwarz, J. P., Spackman, J. R., Perring, A. E., Coe, H., Liu, D., & Clarke, A. D. (2014) · Atmospheric Chemistry and Physics · doi:10.5194/acp-14-10989-2014 · Cited by 323
Metadata
- Authors
- Moteki, N., Kondo, Y., Miyazaki, Y., Takegawa, N., Komazaki, Y., Kurata, G., Shirai, T., Blake, D. R., Miyakawa, T., & Koike, M.
- Venue
- Geophysical Research Letters
- Publisher
- American Geophysical Union (AGU)
- Published
- 2007-06
- Volume
- 34
- Issue
- 11
- ISSN
- 0094-8276 (ISSN-L)
- 1944-8007
- OpenAlex
- W2124958800
- Cited by
- 196
- References
- 0
- FWCI
- 7.11
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Moteki, N., Kondo, Y., Miyazaki, Y., Takegawa, N., Komazaki, Y., Kurata, G., Shirai, T., Blake, D. R., Miyakawa, T., & Koike, M. (2007). Evolution of mixing state of black carbon particles: Aircraft measurements over the western Pacific in March 2004. Geophysical Research Letters. https://doi.org/10.1029/2006gl028943
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