The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
A highly reversible room-temperature lithium metal battery based on crosslinked hairy nanoparticles
Open accessAbstract
Rough electrodeposition, uncontrolled parasitic side-reactions with electrolytes and dendrite-induced short-circuits have hindered development of advanced energy storage technologies based on metallic lithium, sodium and aluminium electrodes. Solid polymer electrolytes and nanoparticle-polymer composites have shown promise as candidates to suppress lithium dendrite growth, but the challenge of simultaneously maintaining high mechanical strength and high ionic conductivity at room temperature has so far been unmet in these materials. Here we report a facile and scalable method of fabricating tough, freestanding membranes that combine the best attributes of solid polymers, nanocomposites and gel-polymer electrolytes. Hairy nanoparticles are employed as multifunctional nodes for polymer crosslinking, which produces mechanically robust membranes that are exceptionally effective in inhibiting dendrite growth in a lithium metal battery. The membranes are also reported to enable stable cycling of lithium batteries paired with conventional intercalating cathodes. Our findings appear to provide an important step towards room-temperature dendrite-free batteries.
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Cites
Armand, M., & Tarascon, J.-M. (2008) · Nature · doi:10.1038/451652a · Cited by 19,612
Alternative energy technologies
Dresselhaus, M. S., & Thomas, I. L. (2001) · Nature · doi:10.1038/35104599 · Cited by 4,894
High rate and stable cycling of lithium metal anode
Qian, J., Henderson, W. A., Xu, W., Bhattacharya, P., Engelhard, M., Borodin, O., & Zhang, J.-G. (2015) · Nature Communications · doi:10.1038/ncomms7362 · Cited by 2,561
Cited by
Reviving the lithium metal anode for high-energy batteries
Lin, D., Liu, Y., & Cui, Y. (2017) · Nature Nanotechnology · doi:10.1038/nnano.2017.16 · Cited by 6,763
Pathways for practical high-energy long-cycling lithium metal batteries
Liu, J., Bao, Z., Cui, Y., Dufek, E. J., Goodenough, J. B., Khalifah, P., Li, Q., Liaw, B. Y., Liu, P., Manthiram, A., et al. (2019) · Nature Energy · doi:10.1038/s41560-019-0338-x · Cited by 3,412
Designing solid-state electrolytes for safe, energy-dense batteries
Zhao, Q., Stalin, S., Zhao, C.-Z., & Archer, L. A. (2020) · Nature Reviews Materials · doi:10.1038/s41578-019-0165-5 · Cited by 2,372
Self-citationDesign principles for electrolytes and interfaces for stable lithium-metal batteries
Tikekar, M. D., Choudhury, S., Tu, Z., & Archer, L. A. (2016) · Nature Energy · doi:10.1038/nenergy.2016.114 · Cited by 1,765
Self-citationPolymer Electrolytes for Lithium-Based Batteries: Advances and Prospects
Zhou, D., Shanmukaraj, D., Tkacheva, A., Armand, M., & Wang, G. (2019) · Chem · doi:10.1016/j.chempr.2019.05.009 · Cited by 1,539
Metadata
- Authors
- Choudhury, S., Mangal, R., Agrawal, A., & Archer, L. A.
- Venue
- Nature Communications
- Published
- 2015-12-04
- Volume
- 6
- Issue
- 1
- Pages
- 10101-10101
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2186290912
- Cited by
- 450
- References
- 3
- FWCI
- 23.58
- Type
- journal article
- Language
- en
- Open access
- gold
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