The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Direct hydrodeoxygenation of raw woody biomass into liquid alkanes
Open accessAbstract
Being the only sustainable source of organic carbon, biomass is playing an ever-increasingly important role in our energy landscape. The conversion of renewable lignocellulosic biomass into liquid fuels is particularly attractive but extremely challenging due to the inertness and complexity of lignocellulose. Here we describe the direct hydrodeoxygenation of raw woods into liquid alkanes with mass yields up to 28.1 wt% over a multifunctional Pt/NbOPO 4 catalyst in cyclohexane. The superior performance of this catalyst allows simultaneous conversion of cellulose, hemicellulose and, more significantly, lignin fractions in the wood sawdust into hexane, pentane and alkylcyclohexanes, respectively. Investigation on the molecular mechanism reveals that a synergistic effect between Pt, NbOx species and acidic sites promotes this highly efficient hydrodeoxygenation of bulk lignocellulose. No chemical pretreatment of the raw woody biomass or separation is required for this one-pot process, which opens a general and energy-efficient route for converting raw lignocellulose into valuable alkanes.
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Cites
Pyrolysis of Wood/Biomass for Bio-oil: A Critical Review
Mohan, D., Pittman, C. U., & Steele, P. H. (2006) · Energy & Fuels · doi:10.1021/ef0502397 · Cited by 5,663
Review of fast pyrolysis of biomass and product upgrading
Bridgwater, A. V. (2012) · Biomass and Bioenergy · doi:10.1016/j.biombioe.2011.01.048 · Cited by 4,856
The Catalytic Valorization of Lignin for the Production of Renewable Chemicals
Zakzeski, J., Bruijnincx, P. C. A., Jongerius, A. L., & Weckhuysen, B. M. (2010) · Chemical Reviews · doi:10.1021/cr900354u · Cited by 4,468
Catalytic conversion of biomass to biofuels
Alonso, D. M., Bond, J. Q., & Dumesic, J. A. (2010) · Green Chemistry · doi:10.1039/c004654j · Cited by 2,333
Cited by
Chemicals from lignin: an interplay of lignocellulose fractionation, depolymerisation, and upgrading
Schutyser, W., Renders, T., Van den Bosch, S., Koelewijn, S.-F., Beckham, G. T., & Sels, B. F. (2018) · Chemical Society Reviews · doi:10.1039/c7cs00566k · Cited by 2,552
Bifunctional Electrocatalysts for Overall and Hybrid Water Splitting
Quan, L., Jiang, H., Mei, G., Sun, Y., & You, B. (2024) · Chemical Reviews · doi:10.1021/acs.chemrev.3c00332 · Cited by 874
Catalytic conversion of lignocellulosic biomass into chemicals and fuels
Deng, W., Feng, Y., Fu, J., Guo, H., Guo, Y., Han, B., Jiang, Z., Kong, L., Li, C., Liu, H., et al. (2023) · Green Energy & Environment · doi:10.1016/j.gee.2022.07.003 · Cited by 854
Self-citationWu, X., Fan, X., Xie, S., Lin, J., Cheng, J., Zhang, Q., Chen, L., & Wang, Y. (2018) · Nature Catalysis · doi:10.1038/s41929-018-0148-8 · Cited by 649
Self-citationSolar-driven reforming of lignocellulose to H2 with a CdS/CdOx photocatalyst
Wakerley, D. W., Kuehnel, M. F., Orchard, K. L., Ly, K. H., Rosser, T. E., & Reisner, E. (2017) · Nature Energy · doi:10.1038/nenergy.2017.21 · Cited by 648
Metadata
- Authors
- Xia, Q., Chen, Z., Shao, Y., Gong, X., Wang, H., Liu, X., Parker, S. F., Han, X., Yang, S., & Wang, Y.
- Venue
- Nature Communications
- Published
- 2016-03-30
- Volume
- 7
- Issue
- 1
- Pages
- 11162-11162
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2322842605
- Cited by
- 464
- References
- 4
- FWCI
- 26.29
- Type
- journal article
- Language
- en
- Open access
- gold
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