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A reversible dendrite-free high-areal-capacity lithium metal electrode
Open accessAbstract
Reversible dendrite-free low-areal-capacity lithium metal electrodes have recently been revived, because of their pivotal role in developing beyond lithium ion batteries. However, there have been no reports of reversible dendrite-free high-areal-capacity lithium metal electrodes. Here we report on a strategy to realize unprecedented stable cycling of lithium electrodeposition/stripping with a highly desirable areal-capacity (12 mAh cm−2) and exceptional Coulombic efficiency (>99.98%) at high current densities (>5 mA cm−2) and ambient temperature using a diluted solvate ionic liquid. The essence of this strategy, that can drastically improve lithium electrodeposition kinetics by cyclic voltammetry premodulation, lies in the tailoring of the top solid-electrolyte interphase layer in a diluted solvate ionic liquid to facilitate a two-dimensional growth mode. We anticipate that this discovery could pave the way for developing reversible dendrite-free metal anodes for sustainable battery chemistries.
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Cites
High rate and stable cycling of lithium metal anode
Qian, J., Henderson, W. A., Xu, W., Bhattacharya, P., Engelhard, M., Borodin, O., & Zhang, J.-G. (2015) · Nature Communications · doi:10.1038/ncomms7362 · Cited by 2,561
Cited by
A facile surface chemistry route to a stabilized lithium metal anode
Liang, X., Pang, Q., Kochetkov, I. R., Sempere, M. S., Huang, H., Sun, X., & Nazar, L. F. (2017) · Nature Energy · doi:10.1038/nenergy.2017.119 · Cited by 1,083
High-energy lithium metal pouch cells with limited anode swelling and long stable cycles
Niu, C., Lee, H., Chen, S., Li, Q., Du, J., Xu, W., Zhang, J.-G., Whittingham, M. S., Xiao, J., & Liu, J. (2019) · Nature Energy · doi:10.1038/s41560-019-0390-6 · Cited by 732
Lithium Metal Anodes with Nonaqueous Electrolytes
Zhang, J.-G., Xu, W., Xiao, J., Cao, X., & Liu, J. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00275 · Cited by 730
Artificial Interphases for Highly Stable Lithium Metal Anode
Xu, R., Cheng, X.-B., Yan, C., Zhang, X.-Q., Xiao, Y., Zhao, C.-Z., Huang, J.-Q., & Zhang, Q. (2019) · Matter · doi:10.1016/j.matt.2019.05.016 · Cited by 721
High-Efficiency Lithium Metal Batteries with Fire-Retardant Electrolytes
Chen, S., Zheng, J., Yu, L., Ren, X., Engelhard, M. H., Niu, C., Lee, H., Xu, W., Xiao, J., Liu, J., et al. (2018) · Joule · doi:10.1016/j.joule.2018.05.002 · Cited by 654
Metadata
- Authors
- Wang, H., Matsui, M., Kuwata, H., Sonoki, H., Matsuda, Y., Shang, X., Takeda, Y., Yamamoto, O., & Imanishi, N.
- Venue
- Nature Communications
- Published
- 2017-04-25
- Volume
- 8
- Issue
- 1
- Pages
- 15106-15106
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2607951315
- Cited by
- 200
- References
- 1
- FWCI
- 10.52
- Type
- journal article
- Language
- en
- Open access
- gold
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- Wang, H., Matsui, M., Kuwata, H., Sonoki, H., Matsuda, Y., Shang, X., Takeda, Y., Yamamoto, O., & Imanishi, N. (2017). A reversible dendrite-free high-areal-capacity lithium metal electrode. Nature Communications. https://doi.org/10.1038/ncomms15106
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