The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Ambipolar zinc-polyiodide electrolyte for a high-energy density aqueous redox flow battery
Open accessAbstract
Redox flow batteries are receiving wide attention for electrochemical energy storage due to their unique architecture and advantages, but progress has so far been limited by their low energy density (~25 Wh l−1). Here we report a high-energy density aqueous zinc-polyiodide flow battery. Using the highly soluble iodide/triiodide redox couple, a discharge energy density of 167 Wh l−1 is demonstrated with a near-neutral 5.0 M ZnI 2 electrolyte. Nuclear magnetic resonance study and density functional theory-based simulation along with flow test data indicate that the addition of an alcohol (ethanol) induces ligand formation between oxygen on the hydroxyl group and the zinc ions, which expands the stable electrolyte temperature window to from −20 to 50 °C, while ameliorating the zinc dendrite. With the high-energy density and its benign nature free from strong acids and corrosive components, zinc-polyiodide flow battery is a promising candidate for various energy storage applications.
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te Velde, G., Bickelhaupt, F. M., Baerends, E. J., Fonseca Guerra, C., van Gisbergen, S. J. A., Snijders, J. G., & Ziegler, T. (2001) · Journal of Computational Chemistry · doi:10.1002/jcc.1056 · Cited by 10,152
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Chu, S., Cui, Y., & Liu, N. (2017) · Nature Materials · doi:10.1038/nmat4834 · Cited by 4,791
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Zhu, Z., Jiang, T., Ali, M., Meng, Y., Jin, Y., Cui, Y., & Chen, W. (2022) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00289 · Cited by 1,769
Redox‐Flow Batteries: From Metals to Organic Redox‐Active Materials
Winsberg, J., Hagemann, T., Janoschka, T., Hager, M. D., & Schubert, U. S. (2017) · Angewandte Chemie International Edition · doi:10.1002/anie.201604925 · Cited by 1,010
A Metal-Organic Framework Host for Highly Reversible Dendrite-free Zinc Metal Anodes
Wang, Z., Huang, J., Guo, Z., Dong, X., Liu, Y., Wang, Y., & Xia, Y. (2019) · Joule · doi:10.1016/j.joule.2019.02.012 · Cited by 938
Towards polyvalent ion batteries: A zinc-ion battery based on NASICON structured Na3V2(PO4)3
Li, G., Yang, Z., Jiang, Y., Jin, C., Huang, W., Ding, X., & Huang, Y. (2016) · Nano Energy · doi:10.1016/j.nanoen.2016.04.051 · Cited by 734
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Metadata
- Authors
- Li, B., Nie, Z., Vijayakumar, M., Li, G., Liu, J., Sprenkle, V., & Wang, W.
- Venue
- Nature Communications
- Published
- 2015-02-24
- Volume
- 6
- Issue
- 1
- Pages
- 6303-6303
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W1965767049
- Cited by
- 604
- References
- 1
- FWCI
- 18.28
- Type
- journal article
- Language
- en
- Open access
- gold
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
