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Low-threshold amplified spontaneous emission and lasing from colloidal nanocrystals of caesium lead halide perovskites
Open accessAbstract
Metal halide semiconductors with perovskite crystal structures have recently emerged as highly promising optoelectronic materials. Despite the recent surge of reports on microcrystalline, thin-film and bulk single-crystalline metal halides, very little is known about the photophysics of metal halides in the form of uniform, size-tunable nanocrystals. Here we report low-threshold amplified spontaneous emission and lasing from ∼10 nm monodisperse colloidal nanocrystals of caesium lead halide perovskites CsPbX 3 (X=Cl, Br or I, or mixed Cl/Br and Br/I systems). We find that room-temperature optical amplification can be obtained in the entire visible spectral range (440–700 nm) with low pump thresholds down to 5±1 μJ cm−2 and high values of modal net gain of at least 450±30 cm−1. Two kinds of lasing modes are successfully observed: whispering-gallery-mode lasing using silica microspheres as high-finesse resonators, conformally coated with CsPbX 3 nanocrystals and random lasing in films of CsPbX 3 nanocrystals.
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Stranks, S. D., Eperon, G. E., Grancini, G., Menelaou, C., Alcocer, M. J. P., Leijtens, T., Herz, L. M., Petrozza, A., & Snaith, H. J. (2013) · Science · doi:10.1126/science.1243982 · Cited by 10,413
Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors
Zhu, H., Fu, Y., Meng, F., Wu, X., Gong, Z., Ding, Q., Gustafsson, M. V., Trinh, M. T., Jin, S., & Zhu, X.-Y. (2015) · Nature Materials · doi:10.1038/nmat4271 · Cited by 2,836
Deschler, F., Price, M., Pathak, S., Klintberg, L. E., Jarausch, D.-D., Higler, R., Hüttner, S., Leijtens, T., Stranks, S. D., Snaith, H. J., et al. (2014) · The Journal of Physical Chemistry Letters · doi:10.1021/jz5005285 · Cited by 1,753
Room-Temperature Near-Infrared High-Q Perovskite Whispering-Gallery Planar Nanolasers
Zhang, Q., Ha, S. T., Liu, X., Sum, T. C., & Xiong, Q. (2014) · Nano Letters · doi:10.1021/nl503057g · Cited by 816
Ultrahigh-Speed Random Number Generation Based on a Chaotic Semiconductor Laser
Reidler, I., Aviad, Y., Rosenbluh, M., & Kanter, I. (2009) · Physical Review Letters · doi:10.1103/physrevlett.103.024102 · Cited by 424
Cited by
Zou, S., Liu, Y., Li, J., Liu, C., Feng, R., Jiang, F., Li, Y., Song, J., Zeng, H., Hong, M., et al. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.7b04000 · Cited by 854
Strongly emissive perovskite nanocrystal inks for high-voltage solar cells
Akkerman, Q. A., Gandini, M., Di Stasio, F., Rastogi, P., Palazon, F., Bertoni, G., Ball, J. M., Prato, M., Petrozza, A., & Manna, L. (2016) · Nature Energy · doi:10.1038/nenergy.2016.194 · Cited by 721
High‐Quality Whispering‐Gallery‐Mode Lasing from Cesium Lead Halide Perovskite Nanoplatelets
Zhang, Q., Su, R., Liu, X., Xing, J., Sum, T. C., & Xiong, Q. (2016) · Advanced Functional Materials · doi:10.1002/adfm.201601690 · Cited by 668
Yettapu, G. R., Talukdar, D., Sarkar, S., Swarnkar, A., Nag, A., Ghosh, P., & Mandal, P. (2016) · Nano Letters · doi:10.1021/acs.nanolett.6b01168 · Cited by 594
Dong, Y., Qiao, T., Kim, D., Parobek, D., Rossi, D., & Son, D. H. (2018) · Nano Letters · doi:10.1021/acs.nanolett.8b00861 · Cited by 580
Metadata
- Authors
- Yakunin, S., Protesescu, L., Krieg, F., Bodnarchuk, M. I., Nedelcu, G., Humer, M., De Luca, G., Fiebig, M., Heiss, W., & Kovalenko, M. V.
- Venue
- Nature Communications
- Published
- 2015-08-20
- Volume
- 6
- Issue
- 1
- Pages
- 8056-8056
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2269917342
- Cited by
- 1,633
- References
- 5
- FWCI
- 79.07
- Type
- journal article
- Language
- en
- Open access
- gold
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- Yakunin, S., Protesescu, L., Krieg, F., Bodnarchuk, M. I., Nedelcu, G., Humer, M., De Luca, G., Fiebig, M., Heiss, W., & Kovalenko, M. V. (2015). Low-threshold amplified spontaneous emission and lasing from colloidal nanocrystals of caesium lead halide perovskites. Nature Communications. https://doi.org/10.1038/ncomms9056
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