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A molecular perspective of water at metal interfaces
Open accessAbstract
Water/solid interfaces are relevant to a broad range of physicochemical phenomena and technological processes such as corrosion, lubrication, heterogeneous catalysis and electrochemistry. Although many fields have contributed to rapid progress in the fundamental knowledge of water at interfaces, detailed molecular-level understanding of water/solid interfaces comes mainly from studies on flat metal substrates. These studies have recently shown that a remarkably rich variety of structures form at the interface between water and even seemingly simple flat surfaces. In this Review we discuss the most exciting work in this area, in particular the emerging physical insight and general concepts about how water binds to metal surfaces. We also provide a perspective on outstanding problems, challenges and open questions.
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Cites
Molecular Structure of Water at Interfaces: Wetting at the Nanometer Scale
Verdaguer, A., Sacha, G. M., Bluhm, H., & Salmeron, M. (2006) · Chemical Reviews · doi:10.1021/cr040376l · Cited by 627
Direct mapping of the solid–liquid adhesion energy with subnanometre resolution
Voïtchovsky, K., Kuna, J. J., Contera, S. A., Tosatti, E., & Stellacci, F. (2010) · Nature Nanotechnology · doi:10.1038/nnano.2010.67 · Cited by 194
Cited by
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Li, C.-Y., Le, J.-B., Wang, Y.-H., Chen, S., Yang, Z.-L., Li, J.-F., Cheng, J., & Tian, Z.-Q. (2019) · Nature Materials · doi:10.1038/s41563-019-0356-x · Cited by 789
The critical role of water at the gold-titania interface in catalytic CO oxidation
Saavedra, J., Doan, H. A., Pursell, C. J., Grabow, L. C., & Chandler, B. D. (2014) · Science · doi:10.1126/science.1256018 · Cited by 608
Tan, H., Tang, B., Lu, Y., Ji, Q., Lv, L., Duan, H., Li, N., Wang, Y., Feng, S., Li, Z., et al. (2022) · Nature Communications · doi:10.1038/s41467-022-29710-w · Cited by 390
The interplay between apparent viscosity and wettability in nanoconfined water
Ortiz-Young, D., Chiu, H.-C., Kim, S., Voïtchovsky, K., & Riedo, E. (2013) · Nature Communications · doi:10.1038/ncomms3482 · Cited by 293
Le, J.-B., Fan, Q.-Y., Li, J.-Q., & Cheng, J. (2020) · Science Advances · doi:10.1126/sciadv.abb1219 · Cited by 269
Metadata
- Authors
- Carrasco, J., Hodgson, A., & Michaelides, A.
- Venue
- Nature Materials
- Published
- 2012-07-24
- Volume
- 11
- Issue
- 8
- Pages
- 667-674
- ISSN
- 1476-1122 (ISSN-L)
- 1476-4660
- OpenAlex
- W1971750100
- Cited by
- 705
- References
- 2
- FWCI
- 18.28
- Type
- journal article
- Language
- en
- Open access
- green
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- Carrasco, J., Hodgson, A., & Michaelides, A. (2012). A molecular perspective of water at metal interfaces. Nature Materials. https://doi.org/10.1038/nmat3354
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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