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Understanding activity trends in electrochemical water oxidation to form hydrogen peroxide
Open accessAbstract
Electrochemical production of hydrogen peroxide (H 2 O 2) from water oxidation could provide a very attractive route to locally produce a chemically valuable product from an abundant resource. Herein using density functional theory calculations, we predict trends in activity for water oxidation towards H 2 O 2 evolution on four different metal oxides, i.e., WO 3, SnO 2, TiO 2 and BiVO 4. The density functional theory predicted trend for H 2 O 2 evolution is further confirmed by our experimental measurements. Moreover, we identify that BiVO 4 has the best H 2 O 2 generation amount of those oxides and can achieve a Faraday efficiency of about 98% for H 2 O 2 production.
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Cites
Origin of the Overpotential for Oxygen Reduction at a Fuel-Cell Cathode
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Self-citationUniversality in Oxygen Evolution Electrocatalysis on Oxide Surfaces
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Self-citationDevelopments and perspectives of oxide-based catalysts for the oxygen evolution reaction
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Tuning selectivity of electrochemical reactions by atomically dispersed platinum catalyst
Choi, C. H., Kim, M., Kwon, H. C., Cho, S. J., Yun, S., Kim, H.-T., Mayrhofer, K. J. J., Kim, H., & Choi, M. (2016) · Nature Communications · doi:10.1038/ncomms10922 · Cited by 849
Sunscreens as a Source of Hydrogen Peroxide Production in Coastal Waters
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Self-citationZnO As an Active and Selective Catalyst for Electrochemical Water Oxidation to Hydrogen Peroxide
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Self-citationDo, V.-H., & Lee, J.-M. (2022) · ACS Nano · doi:10.1021/acsnano.2c08919 · Cited by 292
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Metadata
- Authors
- Shi, X., Siahrostami, S., Li, G.-L., Zhang, Y., Chakthranont, P., Studt, F., Jaramillo, T. F., Zheng, X., & Nørskov, J. K.
- Venue
- Nature Communications
- Published
- 2017-09-26
- Volume
- 8
- Issue
- 1
- Pages
- 701-701
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2755245524
- Cited by
- 541
- References
- 6
- FWCI
- 8.25
- Type
- journal article
- Language
- en
- Open access
- gold
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- Shi, X., Siahrostami, S., Li, G.-L., Zhang, Y., Chakthranont, P., Studt, F., Jaramillo, T. F., Zheng, X., & Nørskov, J. K. (2017). Understanding activity trends in electrochemical water oxidation to form hydrogen peroxide. Nature Communications. https://doi.org/10.1038/s41467-017-00585-6
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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