The DOI matches its Crossref record; 6 of the 6 references it cites were found in a registry or an index.
Half-metallic carbon nitride nanosheets with micro grid mode resonance structure for efficient photocatalytic hydrogen evolution
Open accessAbstract
Photocatalytic hydrogen evolution from water has triggered an intensive search for metal-free semiconducting photocatalysts. However, traditional semiconducting materials suffer from limited hydrogen evolution efficiency owing to low intrinsic electron transfer, rapid recombination of photogenerated carriers, and lack of artificial microstructure. Herein, we report a metal-free half-metallic carbon nitride for highly efficient photocatalytic hydrogen evolution. The introduced half-metallic features not only effectively facilitate carrier transfer but also provide more active sites for hydrogen evolution reaction. The nanosheets incorporated into a micro grid mode resonance structure via in situ pyrolysis of ionic liquid, which show further enhanced photoelectronic coupling and entire solar energy exploitation, boosts the hydrogen evolution rate reach up to 1009 μmol g−1 h−1. Our findings propose a strategy for micro-structural regulations of half-metallic carbon nitride material, and meanwhile the fundamentals provide inspirations for the steering of electron transfer and solar energy absorption in electrocatalysis, photoelectrocatalysis, and photovoltaic cells.
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Non-adiabatic crossing of energy levels
Zener, C. (1932) · Proceedings of the Royal Society of London Series A Containing Papers of a Mathematical and Physical Character · doi:10.1098/rspa.1932.0165 · Cited by 4,572
Metal-free efficient photocatalyst for stable visible water splitting via a two-electron pathway
Liu, J., Liu, Y., Liu, N., Han, Y., Zhang, X., Huang, H., Lifshitz, Y., Lee, S.-T., Zhong, J., & Kang, Z. (2015) · Science · doi:10.1126/science.aaa3145 · Cited by 4,468
Enhanced catalytic activity in strained chemically exfoliated WS2 nanosheets for hydrogen evolution
Voiry, D., Yamaguchi, H., Li, J., Silva, R., Alves, D. C. B., Fujita, T., Chen, M., Asefa, T., Shenoy, V. B., Eda, G., et al. (2013) · Nature Materials · doi:10.1038/nmat3700 · Cited by 2,641
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Self-citationPu, Z., Amiinu, I. S., Kou, Z., Li, W., & Mu, S. (2017) · Angewandte Chemie International Edition · doi:10.1002/anie.201704911 · Cited by 671
Cited by
Metal-free photocatalysts for hydrogen evolution
Rahman, M. Z., Kibria, M. G., & Mullins, C. B. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00313d · Cited by 565
Metadata
- Authors
- Zhou, G., Shan, Y., Hu, Y., Xu, X., Long, L., Zhang, J., Dai, J., Guo, J., Shen, J., Li, S., Liu, L., & Wu, X.
- Venue
- Nature Communications
- Published
- 2018-08-22
- Volume
- 9
- Issue
- 1
- Pages
- 3366-3366
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2887822003
- Cited by
- 275
- References
- 6
- FWCI
- 7.35
- Type
- journal article
- Language
- en
- Open access
- gold
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- Zhou, G., Shan, Y., Hu, Y., Xu, X., Long, L., Zhang, J., Dai, J., Guo, J., Shen, J., Li, S., Liu, L., & Wu, X. (2018). Half-metallic carbon nitride nanosheets with micro grid mode resonance structure for efficient photocatalytic hydrogen evolution. Nature Communications. https://doi.org/10.1038/s41467-018-05590-x
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