The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Two-dimensional transition metal carbides as supports for tuning the chemistry of catalytic nanoparticles
Open accessAbstract
Supported nanoparticles are broadly employed in industrial catalytic processes, where the active sites can be tuned by metal-support interactions (MSIs). Although it is well accepted that supports can modify the chemistry of metal nanoparticles, systematic utilization of MSIs for achieving desired catalytic performance is still challenging. The developments of supports with appropriate chemical properties and identification of the resulting active sites are the main barriers. Here, we develop two-dimensional transition metal carbides (MXenes) supported platinum as efficient catalysts for light alkane dehydrogenations. Ordered Pt 3 Ti and surface Pt 3 Nb intermetallic compound nanoparticles are formed via reactive metal-support interactions on Pt/Ti 3 C 2 Txand Pt/Nb 2 CTxcatalysts, respectively. MXene supports modulate the nature of the active sites, making them highly selective toward C–H activation. Such exploitation of the MSIs makes MXenes promising platforms with versatile chemical reactivity and tunability for facile design of supported intermetallic nanoparticles over a wide range of compositions and structures.
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Cites
Strong metal-support interactions. Group 8 noble metals supported on titanium dioxide
Tauster, S. J., Fung, S. C., & Garten, R. L. (1978) · Journal of the American Chemical Society · doi:10.1021/ja00469a029 · Cited by 3,188
Cited by
Jiang, X., Kuklin, A. V., Baev, A., Ge, Y., Ågren, H., Zhang, H., & Prasad, P. N. (2020) · Physics Reports · doi:10.1016/j.physrep.2019.12.006 · Cited by 914
Propane dehydrogenation: catalyst development, new chemistry, and emerging technologies
Chen, S., Chang, X., Sun, G., Zhang, T., Xu, Y., Wang, Y., Pei, C., & Gong, J. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00814a · Cited by 895
Liu, L., & Corma, A. (2023) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00733 · Cited by 689
Kou, T., Wang, S., Hauser, J. L., Chen, M., Oliver, S. R. J., Ye, Y., Guo, J., & Li, Y. (2019) · ACS Energy Letters · doi:10.1021/acsenergylett.9b00047 · Cited by 314
Zhao, F., Yao, Y., Jiang, C., Shao, Y., Barceló, D., Ying, Y., & Ping, J. (2020) · Journal of Hazardous Materials · doi:10.1016/j.jhazmat.2019.121358 · Cited by 253
Metadata
- Authors
- Li, Z., Yu, L., Milligan, C., Ma, T., Zhou, L., Cui, Y., Qi, Z., Libretto, N., Xu, B., Luo, J., Shi, E., Wu, Z., Xin, H., Delgass, W. N., Miller, J. T., & Wu, Y.
- Venue
- Nature Communications
- Published
- 2018-12-10
- Volume
- 9
- Issue
- 1
- Pages
- 5258-5258
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2902972860
- Cited by
- 270
- References
- 1
- FWCI
- 5.55
- Type
- journal article
- Language
- en
- Open access
- gold
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- Li, Z., Yu, L., Milligan, C., Ma, T., Zhou, L., Cui, Y., Qi, Z., Libretto, N., Xu, B., Luo, J., Shi, E., Wu, Z., Xin, H., Delgass, W. N., Miller, J. T., & Wu, Y. (2018). Two-dimensional transition metal carbides as supports for tuning the chemistry of catalytic nanoparticles. Nature Communications. https://doi.org/10.1038/s41467-018-07502-5
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