The DOI matches its Crossref record; 5 of the 5 references it cites were found in a registry or an index.
The stability of P2-layered sodium transition metal oxides in ambient atmospheres
Open accessAbstract
Air-stability is one of the most important considerations for the practical application of electrode materials in energy-harvesting/storage devices, ranging from solar cells to rechargeable batteries. The promising P2-layered sodium transition metal oxides (P2-Na x TmO 2) often suffer from structural/chemical transformations when contacted with moist air. However, these elaborate transitions and the evaluation rules towards air-stable P2-Na x TmO 2 have not yet been clearly elucidated. Herein, taking P2-Na 0.67 MnO 2 and P2-Na 0.67 Ni 0.33 Mn 0.67 O 2 as key examples, we unveil the comprehensive structural/chemical degradation mechanisms of P2-Na x TmO 2 in different ambient atmospheres by using various microscopic/spectroscopic characterizations and first-principle calculations. The extent of bulk structural/chemical transformation of P2-Na x TmO 2 is determined by the amount of extracted Na+, which is mainly compensated by Na+/H+ exchange. By expanding our study to a series of Mn-based oxides, we reveal that the air-stability of P2-Na x TmO 2 is highly related to their oxidation features in the first charge process and further propose a practical evaluating rule associated with redox couples for air-stable Na x TmO 2 cathodes.
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Cited by
Zuo, W., Innocenti, A., Zarrabeitia, M., Bresser, D., Yang, Y., & Passerini, S. (2023) · Accounts of Chemical Research · doi:10.1021/acs.accounts.2c00690 · Cited by 451
Self-citationZuo, W., Luo, M., Liu, X., Wu, J., Liu, H., Li, J., Winter, M., Fu, R., Yang, W., & Yang, Y. (2020) · Energy & Environmental Science · doi:10.1039/d0ee01694b · Cited by 429
Self-citationElectrochemical energy storage devices working in extreme conditions
Chen, M., Zhang, Y., Xing, G., Chou, S.-L., & Tang, Y. (2021) · Energy & Environmental Science · doi:10.1039/d1ee00271f · Cited by 346
Challenges and industrial perspectives on the development of sodium ion batteries
Cai, X., Yue, Y., Yi, Z., Liu, J., Sheng, Y., & Lu, Y. (2024) · Nano Energy · doi:10.1016/j.nanoen.2024.110052 · Cited by 336
Self-citationChallenges and Prospects of Sodium‐Ion and Potassium‐Ion Batteries for Mass Production
Sada, K., Darga, J., & Manthiram, A. (2023) · Advanced Energy Materials · doi:10.1002/aenm.202302321 · Cited by 308
Metadata
- Authors
- Zuo, W., Qiu, J., Liu, X., Ren, F., Liu, H., He, H., Luo, C., Li, J., Ortiz, G. F., Duan, H., Liu, J., Wang, M.-S., Li, Y., Fu, R., & Yang, Y.
- Venue
- Nature Communications
- Published
- 2020-07-15
- Volume
- 11
- Issue
- 1
- Pages
- 3544-3544
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W3043676137
- Cited by
- 487
- References
- 5
- FWCI
- 15.95
- Type
- journal article
- Language
- en
- Open access
- gold
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- Zuo, W., Qiu, J., Liu, X., Ren, F., Liu, H., He, H., Luo, C., Li, J., Ortiz, G. F., Duan, H., Liu, J., Wang, M.-S., Li, Y., Fu, R., & Yang, Y. (2020). The stability of P2-layered sodium transition metal oxides in ambient atmospheres. Nature Communications. https://doi.org/10.1038/s41467-020-17290-6
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