The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Iron phthalocyanine with coordination induced electronic localization to boost oxygen reduction reaction
Open accessAbstract
Iron phthalocyanine (FePc) is a promising non-precious catalyst for the oxygen reduction reaction (ORR). Unfortunately, FePc with plane-symmetric FeN 4 site usually exhibits an unsatisfactory ORR activity due to its poor O 2 adsorption and activation. Here, we report an axial Fe–O coordination induced electronic localization strategy to improve its O 2 adsorption, activation and thus the ORR performance. Theoretical calculations indicate that the Fe–O coordination evokes the electronic localization among the axial direction of O–FeN 4 sites to enhance O 2 adsorption and activation. To realize this speculation, FePc is coordinated with an oxidized carbon. Synchrotron X-ray absorption and Mössbauer spectra validate Fe–O coordination between FePc and carbon. The obtained catalyst exhibits fast kinetics for O 2 adsorption and activation with an ultralow Tafel slope of 27.5 mV dec−1 and a remarkable half-wave potential of 0.90 V. This work offers a new strategy to regulate catalytic sites for better performance.
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Cites
Generalized Gradient Approximation Made Simple
Perdew, J. P., Burke, K., & Ernzerhof, M. (1996) · Physical Review Letters · doi:10.1103/physrevlett.77.3865 · Cited by 215,824
Projector augmented-wave method
Blöchl, P. E. (1994) · Physical Review B · doi:10.1103/physrevb.50.17953 · Cited by 92,732
Dopant-induced electron localization drives CO2 reduction to C2 hydrocarbons
Zhou, Y., Che, F., Liu, M., Zou, C., Liang, Z., De Luna, P., Yuan, H., Li, J., Wang, Z., Xie, H., et al. (2018) · Nature Chemistry · doi:10.1038/s41557-018-0092-x · Cited by 1,171
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Cited by
Chen, Y., Gao, R., Ji, S., Li, H., Tang, K., Jiang, P., Hu, H., Zhang, Z., Hao, H., Qu, Q., et al. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202012798 · Cited by 650
Self-citationLiu, M., Li, N., Cao, S., Wang, X., Lu, X., Kong, L., Xu, Y., & Bu, X. (2022) · Advanced Materials · doi:10.1002/adma.202107421 · Cited by 341
Self-citationA durable half-metallic diatomic catalyst for efficient oxygen reduction
Li, H., Di, S., Niu, P., Wang, S., Wang, J., & Li, L. (2022) · Energy & Environmental Science · doi:10.1039/d1ee03194e · Cited by 325
Self-citationCai, C., Liu, K., Zhu, Y., Li, P., Wang, Q., Liu, B., Chen, S., Li, H., Zhu, L., Li, H., et al. (2022) · Angewandte Chemie International Edition · doi:10.1002/anie.202113664 · Cited by 213
Self-citationBioinspired and Bioderived Aqueous Electrocatalysis
Barrio, J., Pedersen, A., Favero, S., Luo, H., Wang, M., Sarma, S. C., Feng, J., Ngoc, L. T. T., Kellner, S., Li, A. Y., et al. (2023) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00429 · Cited by 80
Metadata
- Authors
- Chen, K., Liu, K., An, P., Li, H., Lin, Y., Hu, J., Jia, C., Fu, J., Li, H., Liu, H., Lin, Z., Li, W., Li, J., Lu, Y.-R., Chan, T.-S., Zhang, N., & Liu, M.
- Venue
- Nature Communications
- Published
- 2020-08-20
- Volume
- 11
- Issue
- 1
- Pages
- 4173-4173
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W3066041726
- Cited by
- 678
- References
- 3
- FWCI
- 17.73
- Type
- journal article
- Language
- en
- Open access
- gold
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- Chen, K., Liu, K., An, P., Li, H., Lin, Y., Hu, J., Jia, C., Fu, J., Li, H., Liu, H., Lin, Z., Li, W., Li, J., Lu, Y.-R., Chan, T.-S., Zhang, N., & Liu, M. (2020). Iron phthalocyanine with coordination induced electronic localization to boost oxygen reduction reaction. Nature Communications. https://doi.org/10.1038/s41467-020-18062-y
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