The DOI matches its Crossref record; 44 of the 44 references it cites were found in a registry or an index.
In-situ visualization of the space-charge-layer effect on interfacial lithium-ion transport in all-solid-state batteries
Open accessAbstract
The space charge layer (SCL) is generally considered one of the origins of the sluggish interfacial lithium-ion transport in all-solid-state lithium-ion batteries (ASSLIBs). However, in-situ visualization of the SCL effect on the interfacial lithium-ion transport in sulfide-based ASSLIBs is still a great challenge. Here, we directly observe the electrode/electrolyte interface lithium-ion accumulation resulting from the SCL by investigating the net-charge-density distribution across the high-voltage LiCoO 2/argyrodite Li 6 PS 5 Cl interface using the in-situ differential phase contrast scanning transmission electron microscopy (DPC-STEM) technique. Moreover, we further demonstrate a built-in electric field and chemical potential coupling strategy to reduce the SCL formation and boost lithium-ion transport across the electrode/electrolyte interface by the in-situ DPC-STEM technique and finite element method simulations. Our findings will strikingly advance the fundamental scientific understanding of the SCL mechanism in ASSLIBs and shed light on rational electrode/electrolyte interface design for high-rate performance ASSLIBs.
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Cites
A lithium superionic conductor
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A solid future for battery development
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High-power all-solid-state batteries using sulfide superionic conductors
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A review of conduction phenomena in Li-ion batteries
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Self-citationSeino, Y., Ota, T., Takada, K., Hayashi, A., & Tatsumisago, M. (2014) · Energy Environ. Sci. · doi:10.1039/c3ee41655k · Cited by 1,302
Grain-size effects on the ferroelectric behavior of dense nanocrystallineBaTiO3ceramics
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Metadata
- Authors
- Wang, L., Xie, R., Chen, B., Yu, X., Ma, J., Li, C., Hu, Z., Sun, X., Xu, C., Dong, S., Chan, T.-S., Luo, J., Cui, G., & Chen, L.
- Venue
- Nature Communications
- Published
- 2020-11-18
- Volume
- 11
- Issue
- 1
- Pages
- 5889-5889
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W3102869822
- Cited by
- 339
- References
- 44
- FWCI
- 12.32
- Type
- journal article
- Language
- en
- Open access
- gold
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- Wang, L., Xie, R., Chen, B., Yu, X., Ma, J., Li, C., Hu, Z., Sun, X., Xu, C., Dong, S., Chan, T.-S., Luo, J., Cui, G., & Chen, L. (2020). In-situ visualization of the space-charge-layer effect on interfacial lithium-ion transport in all-solid-state batteries. Nature Communications. https://doi.org/10.1038/s41467-020-19726-5
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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