The DOI matches its Crossref record; 47 of the 47 references it cites were found in a registry or an index.
The role of chalcogen vacancies for atomic defect emission in MoS2
Open accessAbstract
For two-dimensional (2D) layered semiconductors, control over atomic defects and understanding of their electronic and optical functionality represent major challenges towards developing a mature semiconductor technology using such materials. Here, we correlate generation, optical spectroscopy, atomic resolution imaging, and ab initio theory of chalcogen vacancies in monolayer MoS 2 . Chalcogen vacancies are selectively generated by in-vacuo annealing, but also focused ion beam exposure. The defect generation rate, atomic imaging and the optical signatures support this claim. We discriminate the narrow linewidth photoluminescence signatures of vacancies, resulting predominantly from localized defect orbitals, from broad luminescence features in the same spectral range, resulting from adsorbates. Vacancies can be patterned with a precision below 10 nm by ion beams, show single photon emission, and open the possibility for advanced defect engineering of 2D semiconductors at the ultimate scale.
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Cited by
2D Materials in Flexible Electronics: Recent Advances and Future Prospectives
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Wang, Y., Sarkar, S., Yan, H., & Chhowalla, M. (2024) · Nature Electronics · doi:10.1038/s41928-024-01210-3 · Cited by 183
Metadata
- Authors
- Mitterreiter, E., Schuler, B., Micevic, A., Hernangómez-Pérez, D., Barthelmi, K., Cochrane, K. A., Kiemle, J., Sigger, F., Klein, J., Wong, E., Barnard, E. S., Watanabe, K., Taniguchi, T., Lorke, M., Jahnke, F., Finley, J. J., Schwartzberg, A. M., Qiu, D. Y., Refaely-Abramson, S., Holleitner, A. W., Weber-Bargioni, A., & Kastl, C.
- Venue
- Nature Communications
- Published
- 2021-06-22
- Volume
- 12
- Issue
- 1
- Pages
- 3822-3822
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W3111360873
- Cited by
- 257
- References
- 47
- FWCI
- 11.35
- Type
- journal article
- Language
- en
- Open access
- gold
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- Mitterreiter, E., Schuler, B., Micevic, A., Hernangómez-Pérez, D., Barthelmi, K., Cochrane, K. A., Kiemle, J., Sigger, F., Klein, J., Wong, E., Barnard, E. S., Watanabe, K., Taniguchi, T., Lorke, M., Jahnke, F., Finley, J. J., Schwartzberg, A. M., Qiu, D. Y., Refaely-Abramson, S., . . . Kastl, C. (2021). The role of chalcogen vacancies for atomic defect emission in MoS2. Nature Communications. https://doi.org/10.1038/s41467-021-24102-y
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