The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Frenkel-defected monolayer MoS2 catalysts for efficient hydrogen evolution
Open accessAbstract
Defect engineering is an effective strategy to improve the activity of two-dimensional molybdenum disulfide base planes toward electrocatalytic hydrogen evolution reaction. Here, we report a Frenkel-defected monolayer MoS 2 catalyst, in which a fraction of Mo atoms in MoS 2 spontaneously leave their places in the lattice, creating vacancies and becoming interstitials by lodging in nearby locations. Unique charge distributions are introduced in the MoS 2 surface planes, and those interstitial Mo atoms are more conducive to H adsorption, thus greatly promoting the HER activity of monolayer MoS 2 base planes. At the current density of 10 mA cm−2, the optimal Frenkel-defected monolayer MoS 2 exhibits a lower overpotential (164 mV) than either pristine monolayer MoS 2 surface plane (358 mV) or Pt-single-atom doped MoS 2 (211 mV). This work provides insights into the structure-property relationship of point-defected MoS 2 and highlights the advantages of Frenkel defects in tuning the catalytic performance of MoS 2 materials.
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Xie, J., Zhang, J., Li, S., Grote, F., Zhang, X., Zhang, H., Wang, R., Lei, Y., Pan, B., & Xie, Y. (2013) · Journal of the American Chemical Society · doi:10.1021/ja408329q · Cited by 2,350
Voiry, D., Fullon, R., Yang, J., de Carvalho Castro e Silva, C., Kappera, R., Bozkurt, I., Kaplan, D., Lagos, M. J., Batson, P. E., Gupta, G., et al. (2016) · Nature Materials · doi:10.1038/nmat4660 · Cited by 824
Ultrahigh-current-density niobium disulfide catalysts for hydrogen evolution
Yang, J., Mohmad, A. R., Wang, Y., Fullon, R., Song, X., Zhao, F., Bozkurt, I., Augustin, M., Santos, E. J. G., Shin, H. S., et al. (2019) · Nature Materials · doi:10.1038/s41563-019-0463-8 · Cited by 401
Cited by
Defect engineering of two-dimensional materials for advanced energy conversion and storage
Liu, F., & Fan, Z. (2023) · Chemical Society Reviews · doi:10.1039/d2cs00931e · Cited by 417
State-of-the-art hydrogen generation techniques and storage methods: A critical review
Tang, D., Tan, G.-L., Li, G.-W., Liang, J.-G., Ahmad, S. M., Bahadur, A., Humayun, M., Ullah, H., Khan, A., & Bououdina, M. (2023) · Journal of Energy Storage · doi:10.1016/j.est.2023.107196 · Cited by 297
2D Transition Metal Dichalcogenides-Based Electrocatalysts for Hydrogen Evolution Reaction
Mondal, A., & Vomiero, A. (2022) · Advanced Functional Materials · doi:10.1002/adfm.202208994 · Cited by 295
Liu, H., Zhang, S., Chai, Y., & Dong, B. (2023) · Angewandte Chemie International Edition · doi:10.1002/anie.202313845 · Cited by 188
Yue, C., Feng, C., Sun, G., Liu, N., Hao, H., Bao, W., Zhang, X., Sun, F., Zhang, C., Bi, J., et al. (2024) · Energy & Environmental Science · doi:10.1039/d3ee04457b · Cited by 125
Metadata
- Authors
- Xu, J., Shao, G., Tang, X., Lv, F., Xiang, H., Jing, C., Liu, S., Dai, S., Li, Y., Luo, J., & Zhou, Z.
- Venue
- Nature Communications
- Published
- 2022-04-22
- Volume
- 13
- Issue
- 1
- Pages
- 2193-2193
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W4224224331
- Cited by
- 378
- References
- 3
- FWCI
- 14.16
- Type
- journal article
- Language
- en
- Open access
- gold
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- Xu, J., Shao, G., Tang, X., Lv, F., Xiang, H., Jing, C., Liu, S., Dai, S., Li, Y., Luo, J., & Zhou, Z. (2022). Frenkel-defected monolayer MoS2 catalysts for efficient hydrogen evolution. Nature Communications. https://doi.org/10.1038/s41467-022-29929-7
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