The DOI matches its Crossref record; 7 of the 7 references it cites were found in a registry or an index.
Anti-dissolution Pt single site with Pt(OH)(O3)/Co(P) coordination for efficient alkaline water splitting electrolyzer
Open accessAbstract
As the most well-known electrocatalyst for cathodic hydrogen evolution in water splitting electrolyzers, platinum is unfortunately inefficient for anodic oxygen evolution due to its over-binding with oxygen species and excessive dissolution in oxidative environment. Herein we show that single Pt atoms dispersed in cobalt hydrogen phosphate with an unique Pt(OH)(O 3)/Co(P) coordination can achieve remarkable catalytic activity and stability for oxygen evolution. The catalyst yields a high turnover frequency (35.1 ± 5.2 s−1) and mass activity (69.5 ± 10.3 A mg−1) at an overpotential of 300 mV and excellent stability. Mechanistic studies elucidate that the superior catalytic performance of isolated Pt atoms herein stems from optimal binding energies of oxygen intermediate and also their strong electronic coupling with neighboring Co atoms that suppresses the formation of soluble Ptx>4 species. Alkaline water electrolyzers assembled with an ultralow Pt loading realizes an industrial-level current density of 1 A cm−2 at 1.8 volts with a high durability.
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Cites
Combining theory and experiment in electrocatalysis: Insights into materials design
Seh, Z. W., Kibsgaard, J., Dickens, C. F., Chorkendorff, I., Nørskov, J. K., & Jaramillo, T. F. (2017) · Science · doi:10.1126/science.aad4998 · Cited by 12,114
Double-slit photoelectron interference in strong-field ionization of the neon dimer
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Universality in Oxygen Evolution Electrocatalysis on Oxide Surfaces
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Homogeneously dispersed multimetal oxygen-evolving catalysts
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Self-citationJiang, K., Liu, B., Luo, M., Ning, S., Peng, M., Zhao, Y., Lu, Y.-R., Chan, T.-S., de Groot, F. M. F., & Tan, Y. (2019) · Nature Communications · doi:10.1038/s41467-019-09765-y · Cited by 670
Mastering the surface strain of platinum catalysts for efficient electrocatalysis
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Zeng, L., Zhao, Z., Huang, Q., Zhou, C., Chen, W., Wang, K., Li, M., Lin, F., Luo, H., Gu, Y., et al. (2023) · Journal of the American Chemical Society · doi:10.1021/jacs.3c06863 · Cited by 325
Self-citationSurface engineering for stable electrocatalysis
Do, V.-H., & Lee, J.-M. (2024) · Chemical Society Reviews · doi:10.1039/d3cs00292f · Cited by 167
Wang, J., Liang, C., Ma, X., Liu, P., Pan, W., Zhu, H., Guo, Z., Sui, Y., Liu, H., Liu, L., et al. (2024) · Advanced Materials · doi:10.1002/adma.202307925 · Cited by 124
Zhou, C., Shi, J., Dong, Z., Zeng, L., Chen, Y., Han, Y., Li, L., Zhang, W., Zhang, Q., Gu, L., et al. (2024) · Nature Communications · doi:10.1038/s41467-024-51200-4 · Cited by 106
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Metadata
- Authors
- Zeng, L., Zhao, Z., Lv, F., Xia, Z., Lu, S.-Y., Li, J., Sun, K., Wang, K., Sun, Y., Huang, Q., Chen, Y., Zhang, Q., Gu, L., Lu, G., & Guo, S.
- Venue
- Nature Communications
- Published
- 2022-07-02
- Volume
- 13
- Issue
- 1
- Pages
- 3822-3822
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W4283784290
- Cited by
- 199
- References
- 7
- FWCI
- 8.15
- Type
- journal article
- Language
- en
- Open access
- gold
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- Zeng, L., Zhao, Z., Lv, F., Xia, Z., Lu, S.-Y., Li, J., Sun, K., Wang, K., Sun, Y., Huang, Q., Chen, Y., Zhang, Q., Gu, L., Lu, G., & Guo, S. (2022). Anti-dissolution Pt single site with Pt(OH)(O3)/Co(P) coordination for efficient alkaline water splitting electrolyzer. Nature Communications. https://doi.org/10.1038/s41467-022-31406-0
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