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Evidence for moiré excitons in van der Waals heterostructures

Open access
Tran, Kha, Moody, Galan, Wu, Fengcheng, Lu, Xiaobo, Choi, Junho, Kim, Kyounghwan, Rai, Amritesh, Sanchez, Daniel A., Quan, Jiamin, Singh, Akshay, Embley, Jacob, Zepeda, André, Campbell, Marshall, Autry, Travis, Taniguchi, Takashi, Watanabe, Kenji, Lu, Nanshu, Banerjee, Sanjay K., Silverman, Kevin L., Kim, Suenne, Tutuc, Emanuel, Yang, Li, MacDonald, Allan H., Li, Xiaoqin·2019·Nature

Abstract

Recent advances in the isolation and stacking of monolayers of van der Waals materials have provided approaches for the preparation of quantum materials in the ultimate two-dimensional limit1,2. In van der Waals heterostructures formed by stacking two monolayer semiconductors, lattice mismatch or rotational misalignment introduces an in-plane moiré superlattice3. It is widely recognized that the moiré superlattice can modulate the electronic band structure of the material and lead to transport properties such as unconventional superconductivity4 and insulating behaviour driven by correlations5–7; however, the influence of the moiré superlattice on optical properties has not been investigated experimentally. Here we report the observation of multiple interlayer exciton resonances with either positive or negative circularly polarized emission in a molybdenum diselenide/tungsten diselenide (MoSe2/WSe2) heterobilayer with a small twist angle. We attribute these resonances to excitonic ground and excited states confined within the moiré potential. This interpretation is supported by recombination dynamics and by the dependence of these interlayer exciton resonances on twist angle and temperature. These results suggest the feasibility of engineering artificial excitonic crystals using van der Waals heterostructures for nanophotonics and quantum information applications. Multiple interlayer exciton resonances in a MoSe2/WSe2 heterobilayer with a small twist angle are attributed to excitonic ground and excited states confined within the moiré potential.

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Metadata

Authors
Tran, K., Moody, G., Wu, F., Lu, X., Choi, J., Kim, K., Rai, A., Sanchez, D. A., Quan, J., Singh, A., Embley, J., Zepeda, A., Campbell, M., Autry, T., Taniguchi, T., Watanabe, K., Lu, N., Banerjee, S. K., Silverman, K. L., Kim, S., Tutuc, E., Yang, L., MacDonald, A. H., & Li, X.
Venue
Nature
Published
2019-02-25
Volume
567
Issue
7746
Pages
71-75
ISSN
  • 0028-0836 (ISSN-L)
  • 1476-4687
OpenAlex
W2916906462
Cited by
1,371
References
42
FWCI
62.61
Type
journal article
Language
en
Open access
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CoChat. (2026). Citation check: Evidence for moiré excitons in van der Waals heterostructures. https://app.cochat.ai/papers/10.1038/s41586-019-0975-z
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Tran, K., Moody, G., Wu, F., Lu, X., Choi, J., Kim, K., Rai, A., Sanchez, D. A., Quan, J., Singh, A., Embley, J., Zepeda, A., Campbell, M., Autry, T., Taniguchi, T., Watanabe, K., Lu, N., Banerjee, S. K., Silverman, K. L., . . . Li, X. (2019). Evidence for moiré excitons in van der Waals heterostructures. Nature. https://doi.org/10.1038/s41586-019-0975-z

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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).

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