Selective electrochemical synthesis of urea from nitrate and CO2 via relay catalysis on hybrid catalysts
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Interfacial spillover offers a promising route to circumvent scaling-relation constraints by spatially separating elementary reaction steps across kinetically optimized components.
“such interfacial spillover offers a promising route to circumvent these constraints by spatially separating elementary reaction steps across kinetically optimized components, thereby enabling each step to proceed under favorable conditions and overcoming activity limitations imposed by scaling relations.21−23”
From High-Entropy Alloy Aerogels with High-Density Solid–Solid Heterointerfaces for Alkaline Hydrogen Evolution (2026) · cites this paper as [22]
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References 33 · Cited by 380
Research works printed but not linked: 2
- Molecule of the Week Archive Ammonia, www.acs.org/content/acs/en/molecule-of-the- week/archive/a/ammonia.html.
- Molecule of the Week Archive Urea, www.acs.org/content/acs/en/molecule-of-the- week/archive/u/urea.html.
- Authors
- Luo, Y., Xie, K., Ou, P., Lavallais, C., Peng, T., Chen, Z., Zhang, Z., Wang, N., Li, X.-Y., Grigioni, I., Liu, B., Sinton, D., Dunn, J. B., & Sargent, E. H.
- Affiliations
- University of Toronto (CA)
- Northwestern University (US)
- Tsinghua–Berkeley Shenzhen Institute (CN)
- Corresponding author
- Dunn, Jennifer B.
- Sargent, Edward H.
- ORCID
- Venue
- Nature Catalysis
- Published
- 2023-09-11
- Volume
- 6
- Issue
- 10
- Pages
- 939-948
- ISSN
- 2520-1158 (ISSN-L)
- OpenAlex
- W4386615148
- Cited by
- 380
- References
- 33
- Citations by year
- 2026: 99 · 2025: 157 · 2024: 123 · 2023: 1
- FWCI
- 18.15
- Type
- journal article
- Language
- en
- Open access
- green
- hdl.handle.net
- Licence
- Locations
- Nature Catalysis (publishedVersion)
- Archivio Istituzionale della Ricerca (Universita Degli Studi Di Milano) (submittedVersion, other-oa)
- TSpace (University of Toronto) (submittedVersion, cc-by-nc-nd)
- Funders
- Salt Science Research Foundation (BL11B)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
- Physical Sciences › Chemical Engineering › Catalysis › Ammonia Synthesis and Nitrogen Reduction
- Physical Sciences › Chemical Engineering › Process Chemistry and Technology › Carbon dioxide utilization in catalysis
- Keywords
- urea electrosynthesis, nitrate reduction, CO2 reduction, relay catalysis, hybrid catalysts, Faradaic efficiency, agricultural runoff, life cycle assessment, greenhouse gas emissions, nitrogen cycling
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