Breaking the linear scaling limit in multi-electron-transfer electrocatalysis through intermediate spillover
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Interfacial spillover offers a promising route to circumvent scaling-relation constraints by spatially separating elementary reaction steps across kinetically optimized components.
“such interfacial spillover offers a promising route to circumvent these constraints by spatially separating elementary reaction steps across kinetically optimized components, thereby enabling each step to proceed under favorable conditions and overcoming activity limitations imposed by scaling relations.21−23”
From High-Entropy Alloy Aerogels with High-Density Solid–Solid Heterointerfaces for Alkaline Hydrogen Evolution (2026) · cites this paper as [21]
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References 72 · Cited by 121
- Authors
- Wang, Q., Hung, S.-F., Lao, K., Huang, X., Li, F., Tao, H. B., Yang, H. B., Liu, W., Wang, W., Cheng, Y., Hiraoka, N., Zhang, L., Zhang, J., Liu, Y., Chen, J., Xu, Y., Su, C., Chen, J. G., & Liu, B.
- Affiliations
- City University of Hong Kong (HK)
- National Yang Ming Chiao Tung University (TW)
- Xiamen University (CN)
- Nanyang Technological University (SG)
- Suzhou University of Science and Technology (CN)
- Dalian Institute of Chemical Physics (CN)
- Dalian University of Technology (CN)
- National Synchrotron Radiation Research Center (TW)
- Chinese Academy of Sciences (CN)
- Zhejiang University of Technology (CN)
- Shenzhen University (CN)
- Corresponding author
- Tao, Hua Bing
- Chen, Jiazang
- Chen, Jingguang G.
- Liu, Bin
- ORCID
- Venue
- Nature Catalysis
- Published
- 2025-04-02
- Volume
- 8
- Issue
- 4
- Pages
- 378-388
- ISSN
- 2520-1158 (ISSN-L)
- OpenAlex
- W4409162162
- Cited by
- 121
- References
- 72
- Citations by year
- 2026: 78 · 2025: 43
- FWCI
- 16.70
- Type
- journal article
- Language
- en
- Open access
- closed
- Licence
- Locations
- Nature Catalysis (publishedVersion)
- DR-NTU (Nanyang Technological University) (submittedVersion)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Materials Science › Materials Chemistry › Catalytic Processes in Materials Science
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
- Keywords
- linear scaling relationship, oxygen reduction reaction, intermediate adsorption energy, oxygen binding energy, half-wave potential, heterogeneous catalysis
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