The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Thermodynamic explanation of the universal correlation between oxygen evolution activity and corrosion of oxide catalysts
Open accessAbstract
In recent years, the oxygen evolution reaction (OER) has attracted increased research interest due to its crucial role in electrochemical energy conversion devices for renewable energy applications. The vast majority of OER catalyst materials investigated are metal oxides of various compositions. The experimental results obtained on such materials strongly suggest the existence of a fundamental and universal correlation between the oxygen evolution activity and the corrosion of metal oxides. This corrosion manifests itself in structural changes and/or dissolution of the material. We prove from basic thermodynamic considerations that any metal oxide must become unstable under oxygen evolution conditions irrespective of the pH value. The reason is the thermodynamic instability of the oxygen anion in the metal oxide lattice. Our findings explain many of the experimentally observed corrosion phenomena on different metal oxide OER catalysts.
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Cites
The Mechanism of Water Oxidation: From Electrolysis via Homogeneous to Biological Catalysis
Dau, H., Limberg, C., Reier, T., Risch, M., Roggan, S., & Strasser, P. (2010) · ChemCatChem · doi:10.1002/cctc.201000126 · Cited by 1,783
Developments and perspectives of oxide-based catalysts for the oxygen evolution reaction
Fabbri, E., Habereder, A., Waltar, K., Kötz, R., & Schmidt, T. J. (2014) · Catal. Sci. Technol. · doi:10.1039/c4cy00669k · Cited by 1,303
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Cited by
A review on fundamentals for designing oxygen evolution electrocatalysts
Song, J., Wei, C., Huang, Z.-F., Liu, C., Zeng, L., Wang, X., & Xu, Z. J. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00607a · Cited by 2,936
Chen, F.-Y., Wu, Z.-Y., Adler, Z., & Wang, H. (2021) · Joule · doi:10.1016/j.joule.2021.05.005 · Cited by 1,284
Reier, T., Nong, H. N., Teschner, D., Schlögl, R., & Strasser, P. (2017) · Advanced Energy Materials · doi:10.1002/aenm.201601275 · Cited by 1,253
Fe-Based Electrocatalysts for Oxygen Evolution Reaction: Progress and Perspectives
Feng, C., Faheem, M. B., Fu, J., Xiao, Y., Li, C., & Li, Y. (2020) · ACS Catalysis · doi:10.1021/acscatal.9b05445 · Cited by 587
Measurement Techniques for the Study of Thin Film Heterogeneous Water Oxidation Electrocatalysts
Stevens, M. B., Enman, L. J., Batchellor, A. S., Cosby, M. R., Vise, A. E., Trang, C. D. M., & Boettcher, S. W. (2017) · Chemistry of Materials · doi:10.1021/acs.chemmater.6b02796 · Cited by 586
Metadata
- Authors
- Binninger, T., Mohamed, R., Waltar, K., Fabbri, E., Levecque, P., Kötz, R., & Schmidt, T. J.
- Venue
- Scientific Reports
- Published
- 2015-07-16
- Volume
- 5
- Issue
- 1
- Pages
- 12167-12167
- ISSN
- 2045-2322 (ISSN-L)
- OpenAlex
- W2257578864
- Cited by
- 476
- References
- 2
- FWCI
- 7.14
- Type
- journal article
- Language
- en
- Open access
- gold
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