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NIR FT Raman spectroscopic study of flame soot
Abstract
During combustion soot goes through different molecular structures. The Raman spectra of flame soot, collected in premixed flames at different flame heights and flame temperatures, were analysed in regard to their structural properties and in comparison with those of disordered graphite. Besides the G- and D-band of disordered graphite, a third Raman band at approximately 1188 cm-1 was observed which was tentatively assigned to mixed s–s bondings or to the C–C and C2C stretching vibration modes of polyene-like structures. The G-band position, the D-band width, and ID/IG intensity ratio describe the graphitic order in the particles. According to this result the graphitic order of the untreated soot particles decreases with decreasing flame temperature and flame height, whereas the size La of the graphitic sheets is nearly constant.
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Cited by
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Bond, T. C., Doherty, S. J., Fahey, D. W., Forster, P. M., Berntsen, T., DeAngelo, B. J., Flanner, M. G., Ghan, S., Kärcher, B., Koch, D., et al. (2013) · Journal of Geophysical Research: Atmospheres · doi:10.1002/jgrd.50171 · Cited by 6,385
Light Absorption by Carbonaceous Particles: An Investigative Review
Bond, T. C., & Bergstrom, R. W. (2006) · Aerosol Science and Technology · doi:10.1080/02786820500421521 · Cited by 2,980
Kouketsu, Y., Mizukami, T., Mori, H., Endo, S., Aoya, M., Hara, H., Nakamura, D., & Wallis, S. (2014) · Island Arc · doi:10.1111/iar.12057 · Cited by 461
N-doped monolithic carbon aerogel electrodes with optimized features for the electrosorption of ions
Rasines, G., Lavela, P., Macías, C., Zafra, M. C., Tirado, J. L., Parra, J. B., & Ania, C. O. (2015) · Carbon · doi:10.1016/j.carbon.2014.11.015 · Cited by 136
Metadata
- Authors
- Dippel, B., Jander, H., & Heintzenberg, J.
- Venue
- Physical Chemistry Chemical Physics
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 1999
- Volume
- 1
- Issue
- 20
- Pages
- 4707-4712
- ISSN
- 1463-9076 (ISSN-L)
- 1463-9084
- OpenAlex
- W2082037236
- Cited by
- 309
- References
- 0
- FWCI
- 0.51
- Type
- journal article
- Language
- en
- Open access
- closed
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