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Electronic and vibrational properties of a MOF-5 metal–organic framework: ZnO quantum dot behaviour
Abstract
UV-Vis DRS and photoluminescence (PL) spectroscopy, combined with excitation selective Raman spectroscopy, allow us to understand the main optical and vibrational properties of a metal-organic MOF-5 framework. A O(2-)Zn(2+)[rightward arrow] O(-)Zn(+) ligand to metal charge transfer transition (LMCT) at 350 nm, testifies that the Zn(4)O(13) cluster behaves as a ZnO quantum dot (QD). The organic part acts as a photon antenna able to efficiently transfer the energy to the inorganic ZnO-like QD part, where an intense emission at 525 nm occurs.
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Cited by
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Kubacka, A., Fernández-García, M., & Colón, G. (2012) · Chemical Reviews · doi:10.1021/cr100454n · Cited by 2,373
Valenzano, L., Civalleri, B., Chavan, S., Bordiga, S., Nilsen, M. H., Jakobsen, S., Lillerud, K. P., & Lamberti, C. (2011) · Chemistry of Materials · doi:10.1021/cm1022882 · Cited by 1,919
Self-citationMetal–organic frameworks as platforms for clean energy
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Metadata
- Authors
- Bordiga, S., Lamberti, C., Ricchiardi, G., Regli, L., Bonino, F., Damin, A., Lillerud, K.-P., Bjorgen, M., & Zecchina, A.
- Venue
- Chem. Commun.
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2004
- Issue
- 20
- Pages
- 2300-2301
- ISSN
- 1359-7345 (ISSN-L)
- 1364-548X
- OpenAlex
- W2092950827
- Cited by
- 524
- References
- 0
- FWCI
- 2.30
- Type
- journal article
- Language
- en
- Open access
- closed
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- Bordiga, S., Lamberti, C., Ricchiardi, G., Regli, L., Bonino, F., Damin, A., Lillerud, K.-P., Bjorgen, M., & Zecchina, A. (2004). Electronic and vibrational properties of a MOF-5 metal–organic framework: ZnO quantum dot behaviour. Chem. Commun. https://doi.org/10.1039/b407246d
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