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Functionalization of polyoxometalates: towards advanced applications in catalysis and materials science
Abstract
Functionalization via covalent grafting of organic functions allows to tune the redox and acid-base properties, and the solubility of polyoxometalates, to enhance their stability and biological activity and to reduce their toxicity, to facilitate their implementation in extended structures and functional devices. We discuss herein the electronic and binding connections, and the various synthesis methodologies. We emphasize on organonitrogen, organosilyl and organophosphonyl derivatives with special attention to synthesis, characterization and potential applications in catalysis and materials science. We also consider the giant molybdenum oxide-based clusters especially the porous capsule-type clusters (Keplerates) which have high relevance to this context.
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Citations
Cited by
Kreutz, J. E., Shukhaev, A., Du, W., Druskin, S., Daugulis, O., & Ismagilov, R. F. (2010) · Journal of the American Chemical Society · doi:10.1021/ja909853x · Cited by 126
Metadata
- Authors
- Proust, A., Thouvenot, R., & Gouzerh, P.
- Venue
- Chemical Communications
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2008
- Issue
- 16
- Pages
- 1837
- ISSN
- 1359-7345 (ISSN-L)
- 1364-548X
- OpenAlex
- W2017557420
- Cited by
- 898
- References
- 0
- FWCI
- 39.41
- Type
- journal article
- Language
- en
- Open access
- closed
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- Proust, A., Thouvenot, R., & Gouzerh, P. (2008). Functionalization of polyoxometalates: towards advanced applications in catalysis and materials science. Chemical Communications. https://doi.org/10.1039/b715502f
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
