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Enzymes in neoteric solvents: From one-phase to multiphase systems
Abstract
Biphasic systems based on neoteric solvents, e.g. ionic liquids (ILs), supercritical carbon dioxide (scCO2), fluorous solvents (FSs) and liquid polymers (LPs), represent interesting alternatives to organic solvents for designing continuous clean biotransformations methods in non-aqueous environments that directly provide pure products. The classical advantages of scCO2– its ability to extract, dissolve and transport chemicals – are complemented by the high catalytic efficiency of enzymes in liquid neoteric solvents (e.g. ILs, LPs or FSs). Enzyme behaviour in scCO2 and ILs, as well as the phase behaviour of ILs/scCO2, are key parameters for carrying out integral green bioprocesses in continuous operation. Experimental approaches, reactor designs and results are discussed in this Critical review.
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Cites
What is a green solvent? A comprehensive framework for the environmental assessment of solvents
Capello, C., Fischer, U., & Hungerbühler, K. (2007) · Green Chemistry · doi:10.1039/b617536h · Cited by 1,917
Cited by
Expanding the organic toolbox: a guide to integrating biocatalysis in synthesis
Clouthier, C. M., & Pelletier, J. N. (2012) · Chemical Society Reviews · doi:10.1039/c2cs15286j · Cited by 358
Enzymatic Synthesis of Biobased Polyesters and Polyamides
Jiang, Y., & Loos, K. (2016) · Polymers · doi:10.3390/polym8070243 · Cited by 257
Metadata
- Authors
- Lozano, P.
- Venue
- Green Chemistry
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2010
- Volume
- 12
- Issue
- 4
- Pages
- 555
- ISSN
- 1463-9262 (ISSN-L)
- 1463-9270
- OpenAlex
- W2062031433
- Cited by
- 178
- References
- 1
- FWCI
- 8.39
- Type
- journal article
- Language
- en
- Open access
- closed
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