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Recipes for enhanced molecular cooling
Abstract
Molecular nanomagnets are considered valid candidates for magnetic refrigeration at low temperatures. Designing these materials for enhanced cooling requires the control and optimization of the quantum properties at the molecular level, in particular: spin ground state, magnetic anisotropy, and presence of low-lying excited spin states. Herein, we present the theoretical framework together with a critical review of recent results, and perspectives for future developments.
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Cited by
Triazoles and tetrazoles: Prime ligands to generate remarkable coordination materials
Aromí, G., Barrios, L. A., Roubeau, O., & Gamez, P. (2011) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2010.10.038 · Cited by 989
Molecule-based magnetic coolers
Zheng, Y.-Z., Zhou, G.-J., Zheng, Z., & Winpenny, R. E. P. (2014) · Chem. Soc. Rev. · doi:10.1039/c3cs60337g · Cited by 578
High-Nuclearity 3d–4f Clusters as Enhanced Magnetic Coolers and Molecular Magnets
Peng, J.-B., Zhang, Q.-C., Kong, X.-J., Zheng, Y.-Z., Ren, Y.-P., Long, L.-S., Huang, R.-B., Zheng, L.-S., & Zheng, Z. (2012) · Journal of the American Chemical Society · doi:10.1021/ja209752z · Cited by 469
Large Magnetocaloric Effect in a Wells–Dawson Type {Ni6Gd6P6} Cage
Zheng, Y., Evangelisti, M., & Winpenny, R. E. P. (2011) · Angewandte Chemie International Edition · doi:10.1002/anie.201008074 · Cited by 299
Self-citationMachine learning guided design of single-molecule magnets for magnetocaloric applications
Holleis, L., Shivaram, B. S., & Balachandran, P. V. (2019) · Applied Physics Letters · doi:10.1063/1.5094553 · Cited by 29
Metadata
- Authors
- Evangelisti, M., & Brechin, E. K.
- Venue
- Dalton Transactions
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2010
- Volume
- 39
- Issue
- 20
- Pages
- 4672
- ISSN
- 1477-9226 (ISSN-L)
- 1477-9234
- OpenAlex
- W2158391865
- Cited by
- 463
- References
- 0
- FWCI
- 17.31
- Type
- journal article
- Language
- en
- Open access
- closed
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