The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Hydrogenolysis of cellulose combining mineral acids and hydrogenation catalysts
Abstract
A catalytic system capable of reaching high performance in the hydrogenolysis of cellulose at low reaction temperature and short reaction times has been developed. Therefore, supported noble metal catalysts based on Pt, Pd and Ru have been combined with dilute mineral acids. A broad variable set in terms of type of noble metal, type of acid, acid concentration and reaction time could be evaluated based on chemical interpretation and supported by a Design of Experiment (DoE) approach. The variables significantly influenced conversion of cellulose, product range and selectivity towards sugar alcohol formation. Thus, at 160 °C, above 60% yield in sugars and sugar alcohols with 84% selectivity at a cellulose conversion of 72% could be reached. Besides, glycerol, propylene glycol, ethylene glycol and methanol were formed as additional valuable by-products leading to an overall carbon utilization above 89%. Furthermore, the concept was successfully transferred to real feedstocks in the form of spruce reaching close to 60% conversion in only one hour reaction time.
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Cites
Beck-Candanedo, S., Roman, M., & Gray, D. G. (2005) · Biomacromolecules · doi:10.1021/bm049300p · Cited by 1,588
Vanoye, L., Fanselow, M., Holbrey, J. D., Atkins, M. P., & Seddon, K. R. (2009) · Green Chemistry · doi:10.1039/b817882h · Cited by 158
Cited by
Conversion of Biomass into Chemicals over Metal Catalysts
Besson, M., Gallezot, P., & Pinel, C. (2014) · Chemical Reviews · doi:10.1021/cr4002269 · Cited by 1,780
Catalytic conversion of lignocellulosic biomass to fine chemicals and fuels
Zhou, C.-H., Xia, X., Lin, C.-X., Tong, D.-S., & Beltramini, J. (2011) · Chemical Society Reviews · doi:10.1039/c1cs15124j · Cited by 1,420
Catalytic conversion of lignocellulosic biomass into chemicals and fuels
Deng, W., Feng, Y., Fu, J., Guo, H., Guo, Y., Han, B., Jiang, Z., Kong, L., Li, C., Liu, H., et al. (2023) · Green Energy & Environment · doi:10.1016/j.gee.2022.07.003 · Cited by 854
Hydrogenolysis Goes Bio: From Carbohydrates and Sugar Alcohols to Platform Chemicals
Ruppert, A. M., Weinberg, K., & Palkovits, R. (2012) · Angewandte Chemie International Edition · doi:10.1002/anie.201105125 · Cited by 836
Self-citationWang, C., Zhang, X., Liu, Q., Zhang, Q., Chen, L., & Ma, L. (2020) · Fuel Processing Technology · doi:10.1016/j.fuproc.2020.106485 · Cited by 157
Metadata
- Authors
- Palkovits, R., Tajvidi, K., Procelewska, J., Rinaldi, R., & Ruppert, A.
- Venue
- Green Chemistry
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2010
- Volume
- 12
- Issue
- 6
- Pages
- 972
- ISSN
- 1463-9262 (ISSN-L)
- 1463-9270
- OpenAlex
- W1992994440
- Cited by
- 249
- References
- 2
- FWCI
- 13.11
- Type
- journal article
- Language
- en
- Open access
- closed
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- Palkovits, R., Tajvidi, K., Procelewska, J., Rinaldi, R., & Ruppert, A. (2010). Hydrogenolysis of cellulose combining mineral acids and hydrogenation catalysts. Green Chemistry. https://doi.org/10.1039/c000075b
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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