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Oxygen reduction reaction catalyst on lithium/air battery discharge performance
Abstract
Lithium/air batteries have the potential to substantially outperform the best battery system nowadays on the market. Oxygen reduction reaction (ORR) at the cathode in an aprotic organic lithium electrolyte is well-known to limit the discharge rate and capacity of the lithium/air batteries. In this study, the discharge characteristics of Li/air cells with cathodes made of different carbon materials were examined. The results showed that the ORR kinetics in the lithium/air batteries can be drastically improved by using an effective catalyst, achieving higher discharge voltage and rate. The discharge capacity of the lithium/air battery was found to be correlated to the cathode pore volume, to which the mesopore volume of the carbon material has a large contribution. An ORR mechanistic model involving a reaction product deactivating the catalytic sites on the carbon surface is proposed to explain the experimental results.
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Cited by
Chabot, V., Higgins, D., Yu, A., Xiao, X., Chen, Z., & Zhang, J. (2014) · Energy & Environmental Science · doi:10.1039/c3ee43385d · Cited by 1,119
Metal–Air Batteries: Will They Be the Future Electrochemical Energy Storage Device of Choice?
Li, Y., & Lu, J. (2017) · ACS Energy Letters · doi:10.1021/acsenergylett.7b00119 · Cited by 990
Graphene and Graphene‐Based Materials for Energy Storage Applications
Zhu, J., Yang, D., Yin, Z., Yan, Q., & Zhang, H. (2014) · Small · doi:10.1002/smll.201303202 · Cited by 825
Porous electrode materials for lithium-ion batteries–how to prepare them and what makes them special
Vu, A., Qian, Y., & Stein, A. (2012) · Advanced Energy Materials · doi:10.1002/aenm.201200320 · Cited by 719
Pulsed Laser in Liquids Made Nanomaterials for Catalysis
Forsythe, R. C., Cox, C. P., Wilsey, M. K., & Müller, A. M. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.0c01069 · Cited by 259
Metadata
- Authors
- Ren, X., Zhang, S. S., Tran, D. T., & Read, J.
- Venue
- Journal of Materials Chemistry
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2011
- Volume
- 21
- Issue
- 27
- Pages
- 10118
- ISSN
- 0959-9428 (ISSN-L)
- 1364-5501
- OpenAlex
- W1965004023
- Cited by
- 236
- References
- 0
- FWCI
- 20.72
- Type
- journal article
- Language
- en
- Open access
- closed
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- Ren, X., Zhang, S. S., Tran, D. T., & Read, J. (2011). Oxygen reduction reaction catalyst on lithium/air battery discharge performance. Journal of Materials Chemistry. https://doi.org/10.1039/c0jm04170j
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