Gram-scale, low-cost, rapid synthesis of highly stable Mg–ACC nanoparticles and their long-term preservation
Abstract
A simple chemistry route is reported for the gram-scale, low-cost, rapid synthesis of highly stable Mg-ACC nanoparticles. The possible structure of Mg-ACC can be defined as Mg₀.₁₅Ca₀.₈₅CO₃·H₂O₀.₈₅. The molar ratio of Mg²(+):Ca²(+):CO₃²⁻and the concentrations of the reactants (CaCl₂, Na₂CO₃, and MgCl₂) play important roles in the Mg:Ca molar ratio of the obtained Mg-ACC nanoparticles. In particular, Mg-ACC can be preserved for over one year without crystallization by either storing its dry powder at -5°C or storing it in ethanol at 5°C. The ability to synthesize Mg-ACC nanoparticles on a large scale is useful for biomineralization studies and industrial applications.
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The stabilizing effect of Mg in ACC can be attributed to hydrated Mg within the framework of the Mg-ACC nanostructure, which retards proto-dolomite nucleation due to its slow dehydration kinetics.
“This stabilizing effect of Mg in ACC can be attributed to the presence of hydrated Mg within the framework of the Mg-ACC nanostructure, which retards proto-dolomite nucleation due to its slow dehydration kinetics (Raiteri and Gale 2010; Jiang et al. 2010).”
From A route for the direct crystallization of dolomite (2015) · cites this paper as Jiang et al. 2010
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References 28 · Cited by 63
- Authors
- Jiang, J., Gao, M.-R., Qiu, Y.-H., & Yu, S.-H.
- Affiliations
- University of Science and Technology of China (CN)
- Corresponding author
- Yu, Shu-Hong
- Venue
- Nanoscale
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2010
- Volume
- 2
- Issue
- 11
- Pages
- 2358
- ISSN
- 2040-3364 (ISSN-L)
- 2040-3372
- OpenAlex
- W2145405966
- Cited by
- 63
- References
- 28
- Citations by year
- 2026: 2 · 2025: 1 · 2024: 8 · 2023: 3 · 2022: 5 · 2021: 1 · 2020: 4 · 2019: 6 · 2018: 3 · 2017: 4 · 2016: 3 · 2015: 4 · 2014: 7 · 2013: 4 · 2012: 4
- FWCI
- 1.59
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Nanoscale (publishedVersion)
- PubMed (publishedVersion)
- Topics
- Physical Sciences › Materials Science › Biomaterials › Calcium Carbonate Crystallization and Inhibition
- Physical Sciences › Environmental Science › Environmental Engineering › CO2 Sequestration and Geologic Interactions
- Physical Sciences › Environmental Science › Environmental Engineering › Microbial Applications in Construction Materials
- Keywords
- nanoparticle synthesis, gram-scale synthesis, low-cost synthesis, crystallization stability, long-term storage, biomineralization, calcium carbonate
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