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Aerobic oxidation of 5-hydroxylmethylfurfural with homogeneous and nanoparticulate catalysts
Abstract
The aerobic oxidation of 5-hydroxymethylfurfural (HMF) with homogeneous Co(OAc)2/Zn(OAc)2/Br−, and heterogeneous Au–TiO2 and Au–CeO2 nanoparticulate catalysts was carried out in acetic acid with and without a trifluoroacetic acid (HTFA) additive. The selectivity of the oxidation products, 2,5-furandicarboxylic acid (FDCA) and 5-formyl-2-furancarboxylic acid (FFCA), improved in the presence of the HTFA (1 wt%) additive. The homogeneous oxidation catalyst gave higher selectivity for FDCA (60% yield) under 1 atm of O2 at 90 °C while Au–TiO2 afforded 80% FFCA under the same conditions.
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Cited by
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van Putten, R.-J., van der Waal, J. C., de Jong, E., Rasrendra, C. B., Heeres, H. J., & de Vries, J. G. (2013) · Chemical Reviews · doi:10.1021/cr300182k · Cited by 2,886
Conversion of Biomass into Chemicals over Metal Catalysts
Besson, M., Gallezot, P., & Pinel, C. (2014) · Chemical Reviews · doi:10.1021/cr4002269 · Cited by 1,780
Alternative Monomers Based on Lignocellulose and Their Use for Polymer Production
Delidovich, I., Hausoul, P. J. C., Deng, L., Pfützenreuter, R., Rose, M., & Palkovits, R. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00354 · Cited by 773
Catalytic oxidation of carbohydrates into organic acids and furan chemicals
Zhang, Z., & Huber, G. W. (2018) · Chemical Society Reviews · doi:10.1039/c7cs00213k · Cited by 689
Recent Advances in the Catalytic Synthesis of 2,5-Furandicarboxylic Acid and Its Derivatives
Zhang, Z., & Deng, K. (2015) · ACS Catalysis · doi:10.1021/acscatal.5b01491 · Cited by 641
Metadata
- Authors
- Saha, B., Dutta, S., & Abu-Omar, M. M.
- Venue
- Catal. Sci. Technol.
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2012
- Volume
- 2
- Issue
- 1
- Pages
- 79-81
- ISSN
- 2044-4753 (ISSN-L)
- 2044-4761
- OpenAlex
- W2115858808
- Cited by
- 161
- References
- 0
- FWCI
- 5.83
- Type
- journal article
- Language
- en
- Open access
- closed
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- Saha, B., Dutta, S., & Abu-Omar, M. M. (2012). Aerobic oxidation of 5-hydroxylmethylfurfural with homogeneous and nanoparticulate catalysts. Catal. Sci. Technol. https://doi.org/10.1039/c1cy00321f
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