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Photocatalytic oxidation of thiophene on BiVO4with dual co-catalysts Pt and RuO2under visible light irradiation using molecular oxygen as oxidant
Abstract
Thiophene is one of the main sulfur-containing compounds in gasoline and difficult to be oxidized with the conventional oxidative processes. Herein for the first time we report that thiophene can be oxidized to SO3 on BiVO4 co-loaded with Pt and RuO2 co-catalysts (denoted as Pt-RuO2/BiVO4) under visible light irradiation with molecular oxygen as oxidant. The high activity of the catalyst can be achieved by only loading as low as 0.03 wt% of Pt and 0.01 wt% of RuO2 as dual co-catalysts on BiVO4. ESR measurements give the evidence that the active oxygen species (˙OH and O2˙−) generated by photocatalytic processes are involved in the photocatalytic oxidation of thiophene. The considerable enhancement of photocatalytic activity can be attributed to the simultaneous presence of the reduction and oxidation co-catalysts which are beneficial for the efficient separation and transfer of the photo-generated electrons and holes.
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Photocatalysis on TiO2 Surfaces: Principles, Mechanisms, and Selected Results
Linsebigler, A. L., Lu, G., & Yates, J. T. (1995) · Chemical Reviews · doi:10.1021/cr00035a013 · Cited by 11,575
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Roles of Cocatalysts in Photocatalysis and Photoelectrocatalysis
Yang, J., Wang, D., Han, H., & Li, C. (2013) · Accounts of Chemical Research · doi:10.1021/ar300227e · Cited by 2,848
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Metadata
- Authors
- Lin, F., Wang, D., Jiang, Z., Ma, Y., Li, J., Li, R., & Li, C.
- Venue
- Energy Environ. Sci.
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2012
- Volume
- 5
- Issue
- 4
- Pages
- 6400-6406
- ISSN
- 1754-5692 (ISSN-L)
- 1754-5706
- OpenAlex
- W1979797706
- Cited by
- 230
- References
- 1
- FWCI
- 3.81
- Type
- journal article
- Language
- en
- Open access
- closed
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- Lin, F., Wang, D., Jiang, Z., Ma, Y., Li, J., Li, R., & Li, C. (2012). Photocatalytic oxidation of thiophene on BiVO4with dual co-catalysts Pt and RuO2under visible light irradiation using molecular oxygen as oxidant. Energy Environ. Sci. https://doi.org/10.1039/c1ee02880d
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