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Commercial metal–organic frameworks as heterogeneous catalysts
Open accessAbstract
Metal-organic frameworks (MOFs) are porous crystalline materials that have promising applications as heterogeneous catalysts. After describing the composition, textural properties and crystal structure of four commercially available MOFs, we summarize organic transformations for which these commercial MOFs exhibit higher catalytic activity than the corresponding soluble metal salts or metal ion-exchanged zeolites. In the present article, we have focused on reactions requiring Lewis-acid sites or redox centers to illustrate the potential applications and limitations of commercial MOFs. In a final section, we provide our views on future developments whose ultimate target will be the use of a commercial MOF as a heterogeneous catalyst for a real industrial process in fine chemistry, thus, realizing the advantages of these materials with respect to zeolites or other solid catalysts in liquid-phase reactions.
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Cites
Metal-organic framework materials as catalysts
Lee, J., Farha, O. K., Roberts, J., Scheidt, K. A., Nguyen, S. T., & Hupp, J. T. (2009) · Chemical Society Reviews · doi:10.1039/b807080f · Cited by 7,969
Supported gold nanoparticles as catalysts for organic reactions
Corma, A., & Garcia, H. (2008) · Chemical Society Reviews · doi:10.1039/b707314n · Cited by 1,883
Cited by
CO2 Capture and Separations Using MOFs: Computational and Experimental Studies
Yu, J., Xie, L.-H., Li, J.-R., Ma, Y., Seminario, J. M., & Balbuena, P. B. (2017) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00626 · Cited by 1,047
Modified metal-organic frameworks as photocatalysts
Qiu, J., Zhang, X., Feng, Y., Zhang, X., Wang, H., & Yao, J. (2018) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2018.03.039 · Cited by 499
Structuring adsorbents and catalysts by processing of porous powders
Akhtar, F., Andersson, L., Ogunwumi, S., Hedin, N., & Bergström, L. (2014) · Journal of the European Ceramic Society · doi:10.1016/j.jeurceramsoc.2014.01.008 · Cited by 363
Ionic metal-organic frameworks (iMOFs): Design principles and applications
Karmakar, A., Desai, A. V., & Ghosh, S. K. (2016) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2015.08.007 · Cited by 308
Metal organic frameworks as heterogeneous catalysts for the production of fine chemicals
Dhakshinamoorthy, A., Opanasenko, M., Čejka, J., & Garcia, H. (2013) · Catalysis Science & Technology · doi:10.1039/c3cy00350g · Cited by 296
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Metadata
- Authors
- Dhakshinamoorthy, A., Alvaro, M., & Garcia, H.
- Venue
- Chemical Communications
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2012
- Volume
- 48
- Issue
- 92
- Pages
- 11275
- ISSN
- 1359-7345 (ISSN-L)
- 1364-548X
- OpenAlex
- W1995443810
- Cited by
- 422
- References
- 2
- FWCI
- 19.75
- Type
- journal article
- Language
- en
- Open access
- green
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