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Atomic layer deposition of vanadium oxide on carbon nanotubes for high-power supercapacitor electrodes
Abstract
Vanadium oxides may offer high pseudocapacitance but limited electrical conductivity and specific surface area. Atomic layer deposition allowed uniform deposition of smooth nanostructured vanadium oxide coatings on the surface of multi-walled carbon nanotube (MWCNT) electrodes, thus offering a novel route for the formation of binder-free flexible composite electrode fabric for supercapacitor applications with large thickness, controlled porosity, greatly improved electrical conductivity and cycle stability. Electrochemical measurements revealed stable performance of the selected MWCNT–vanadium oxide electrodes and remarkable capacitance of up to ∼1550 F g−1 per active mass of the vanadium oxide and up to ∼600 F g−1 per mass of the composite electrode, significantly exceeding specific capacitance of commercially used activated carbons (100–150 F g−1). Electrochemical performance of the oxide layers was found to strongly depend on the coating thickness.
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Cites
Electrically conductive oxide aerogels: new materials in electrochemistry
Rolison, D. R., & Dunn, B. (2001) · Journal of Materials Chemistry · doi:10.1039/b007591o · Cited by 357
Cited by
Li, Z., Xu, Z., Tan, X., Wang, H., Holt, C. M. B., Stephenson, T., Olsen, B. C., & Mitlin, D. (2013) · Energy & Environmental Science · doi:10.1039/c2ee23599d · Cited by 1,054
Expanded hydrated vanadate for high-performance aqueous zinc-ion batteries
Liu, C., Neale, Z., Zheng, J., Jia, X., Huang, J., Yan, M., Tian, M., Wang, M., Yang, J., & Cao, G. (2019) · Energy & Environmental Science · doi:10.1039/c9ee00956f · Cited by 804
A review of Raman spectroscopy of vanadium oxides
Shvets, P., Dikaya, O., Maksimova, K., & Goikhman, A. (2019) · Journal of Raman Spectroscopy · doi:10.1002/jrs.5616 · Cited by 561
Sun, W., Gao, G., Du, Y., Zhang, K., & Wu, G. (2018) · Journal of Materials Chemistry A · doi:10.1039/c8ta01448e · Cited by 83
Metadata
- Authors
- Boukhalfa, S., Evanoff, K., & Yushin, G.
- Venue
- Energy & Environmental Science
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2012
- Volume
- 5
- Issue
- 5
- Pages
- 6872
- ISSN
- 1754-5692 (ISSN-L)
- 1754-5706
- OpenAlex
- W2026029417
- Cited by
- 499
- References
- 1
- FWCI
- 16.27
- Type
- journal article
- Language
- en
- Open access
- closed
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