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Corrosion of magnesium electrolytes: chlorides – the culprit
Abstract
Chloride containing magnesium electrolytes are corrosive towards non noble metals. Currently the development of non-corrosive magnesium electrolytes is a key challenge on the road to a rechargeable magnesium battery. The component responsible for corrosion of magnesium electrolytes has not been previously elucidated. Here we clarify that chlorides in the cation (Mg2(μ-Cl)3·6THF)+ are a major culprit for corrosion. We also corroborate the feasibility of ion exchange reactions as a suitable synthetic approach towards magnesium electrolytes which do not contain the cation (Mg2(μ-Cl)3·6THF)+. Our results indicate that magnesium organoborates are an interesting class of magnesium electrolytes which undergo magnesium deposition and dissolution and are non-corrosive in nature at high voltages.
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Opportunities and challenges for a sustainable energy future
Chu, S., & Majumdar, A. (2012) · Nature · doi:10.1038/nature11475 · Cited by 12,550
Cited by
Quest for Nonaqueous Multivalent Secondary Batteries: Magnesium and Beyond
Muldoon, J., Bucur, C. B., & Gregory, T. (2014) · Chemical Reviews · doi:10.1021/cr500049y · Cited by 1,376
Self-citationMagnesium–sulfur battery: Its beginning and recent progress
Zhirong, Z.-K., & Maximilian, F. (2017) · MRS Communications · doi:10.1557/mrc.2017.101 · Cited by 90
Metadata
- Authors
- Muldoon, J., Bucur, C. B., Oliver, A. G., Zajicek, J., Allred, G. D., & Boggess, W. C.
- Venue
- Energy Environ. Sci.
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2013
- Volume
- 6
- Issue
- 2
- Pages
- 482-487
- ISSN
- 1754-5692 (ISSN-L)
- 1754-5706
- OpenAlex
- W2091106185
- Cited by
- 231
- References
- 1
- FWCI
- 6.31
- Type
- journal article
- Language
- en
- Open access
- closed
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- Muldoon, J., Bucur, C. B., Oliver, A. G., Zajicek, J., Allred, G. D., & Boggess, W. C. (2013). Corrosion of magnesium electrolytes: chlorides – the culprit. Energy Environ. Sci. https://doi.org/10.1039/c2ee23686a
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